Збережено в:
Бібліографічні деталі
Автори: Dumont, Guillaume, Boulanger, Paul, Côté, Michel, Ernzerhof, Matthias
Формат: Preprint
Опубліковано: 2010
Предмети:
Онлайн доступ:https://arxiv.org/abs/1002.1825
Теги: Додати тег
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Зміст:
  • We present a first-principles study of Peierls distortions in \emph{trans}-polyacetylene, polyacene, and armchair $(n,n)$ carbon nanotubes. Our findings suggest that the ground-state geometries of armchair $(n,n)$ carbon nanotubes, with $n$ up to 6, exhibit a Peierls distortion as it is found for \emph{trans}-polyactetylene. In contrast to previous studies in which no Peierls distortion is found with conventional local and semi-local density functionals, we use a hybrid functional whose exact-exchange admixture has been specifically optimized for the problem at hand.