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Main Authors: Grzesik, Jakob M., Catanzaro, Dominic, Roques-Carmes, Charles, Rosenthal, Eric I., van de Stolpe, Guido L., Karnieli, Aviv, Scuri, Giovanni, Biswas, Souvik, Leedle, Kenneth J., Black, Dylan S., Byer, Robert L., Kaminer, Ido, England, R. Joel, Fan, Shanhui, Solgaard, Olav, Vučković, Jelena
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2508.13112
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author Grzesik, Jakob M.
Catanzaro, Dominic
Roques-Carmes, Charles
Rosenthal, Eric I.
van de Stolpe, Guido L.
Karnieli, Aviv
Scuri, Giovanni
Biswas, Souvik
Leedle, Kenneth J.
Black, Dylan S.
Byer, Robert L.
Kaminer, Ido
England, R. Joel
Fan, Shanhui
Solgaard, Olav
Vučković, Jelena
author_facet Grzesik, Jakob M.
Catanzaro, Dominic
Roques-Carmes, Charles
Rosenthal, Eric I.
van de Stolpe, Guido L.
Karnieli, Aviv
Scuri, Giovanni
Biswas, Souvik
Leedle, Kenneth J.
Black, Dylan S.
Byer, Robert L.
Kaminer, Ido
England, R. Joel
Fan, Shanhui
Solgaard, Olav
Vučković, Jelena
contents Scattering experiments with energetic particles, such as free electrons, have been historically used to reveal the quantum structure of matter. However, realizing coherent interactions between free-electron beams and solid-state quantum systems has remained out of reach, owing to their intrinsically weak coupling. Realizing such coherent control would open up opportunities for hybrid quantum platforms combining free electrons and solid-state qubits for coincident quantum information processing and nanoscale sensing. Here, we present a framework that employs negatively charged nitrogen-vacancy centers (NV-) in diamond as quantum sensors of a bunched electron beam. We develop a Lindblad master equation description of the magnetic free-electron--qubit interactions and identify spin relaxometry as a sensitive probe of the interaction. Experimentally, we integrate a confocal fluorescence microscopy setup into a microwave-bunched electron beam line. We monitor charge-state dynamics and assess their impact on key sensing performance metrics (such as spin readout contrast), defining safe operating parameters for quantum sensing experiments. By performing $T_1$ relaxometry under controlled electron beam exposure, we establish an upper bound on the free-electron--spin coupling strength. Our results establish NV- centers as quantitative probes of free electrons, providing a metrological benchmark for free-electron--qubit coupling under realistic conditions, and chart a route toward solid-state quantum control with electron beams.
format Preprint
id arxiv_https___arxiv_org_abs_2508_13112
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Quantum sensing of electron beams using solid-state spins
Grzesik, Jakob M.
Catanzaro, Dominic
Roques-Carmes, Charles
Rosenthal, Eric I.
van de Stolpe, Guido L.
Karnieli, Aviv
Scuri, Giovanni
Biswas, Souvik
Leedle, Kenneth J.
Black, Dylan S.
Byer, Robert L.
Kaminer, Ido
England, R. Joel
Fan, Shanhui
Solgaard, Olav
Vučković, Jelena
Quantum Physics
Accelerator Physics
Optics
Scattering experiments with energetic particles, such as free electrons, have been historically used to reveal the quantum structure of matter. However, realizing coherent interactions between free-electron beams and solid-state quantum systems has remained out of reach, owing to their intrinsically weak coupling. Realizing such coherent control would open up opportunities for hybrid quantum platforms combining free electrons and solid-state qubits for coincident quantum information processing and nanoscale sensing. Here, we present a framework that employs negatively charged nitrogen-vacancy centers (NV-) in diamond as quantum sensors of a bunched electron beam. We develop a Lindblad master equation description of the magnetic free-electron--qubit interactions and identify spin relaxometry as a sensitive probe of the interaction. Experimentally, we integrate a confocal fluorescence microscopy setup into a microwave-bunched electron beam line. We monitor charge-state dynamics and assess their impact on key sensing performance metrics (such as spin readout contrast), defining safe operating parameters for quantum sensing experiments. By performing $T_1$ relaxometry under controlled electron beam exposure, we establish an upper bound on the free-electron--spin coupling strength. Our results establish NV- centers as quantitative probes of free electrons, providing a metrological benchmark for free-electron--qubit coupling under realistic conditions, and chart a route toward solid-state quantum control with electron beams.
title Quantum sensing of electron beams using solid-state spins
topic Quantum Physics
Accelerator Physics
Optics
url https://arxiv.org/abs/2508.13112