Conformational properties of active semiflexible polymers

Fuente: arXiv
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Hauptverfasser: Eisenstecken, Thomas, Gompper, Gerhard, Winkler, Roland G.
Format: Preprint
Veröffentlicht: 2016
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author Eisenstecken, Thomas
Gompper, Gerhard
Winkler, Roland G.
author_facet Eisenstecken, Thomas
Gompper, Gerhard
Winkler, Roland G.
contents The conformational properties of flexible and semiflexible polymers exposed to active noise are studied theoretically. The noise may originate from the interaction of the polymer with surround- ing active (Brownian) particles or from the inherent motion of the polymer itself, which may be composed of active Brownian particles. In the latter case, the respective monomers are indepen- dently propelled in directions changing diffusively. For the description of the polymer, we adopt the continuous Gaussian semiflexible polymer model. Specifically, the finite polymer extensibility is taken into account which turns out to be essentially for the polymer conformations. Our analytical calculations predict a strong dependence of the relaxation times on the activity. In particular, semi- flexible polymers exhibit a crossover from a bending-elasticity-dominated to the flexible-polymer dynamics with increasing activity. This leads to a significant noise-induced polymer shrinkage over a large range of self-propulsion velocities. For large activities, the polymers swell and their extension becomes comparable to the contour length. The scaling properties of the mean square end-to-end distance with respect to the polymer length and monomer activity are discussed.
format Preprint
id arxiv_https___arxiv_org_abs_1610_07974
institution arXiv
publishDate 2016
record_format arxiv
spellingShingle Conformational properties of active semiflexible polymers
Eisenstecken, Thomas
Gompper, Gerhard
Winkler, Roland G.
Soft Condensed Matter
The conformational properties of flexible and semiflexible polymers exposed to active noise are studied theoretically. The noise may originate from the interaction of the polymer with surround- ing active (Brownian) particles or from the inherent motion of the polymer itself, which may be composed of active Brownian particles. In the latter case, the respective monomers are indepen- dently propelled in directions changing diffusively. For the description of the polymer, we adopt the continuous Gaussian semiflexible polymer model. Specifically, the finite polymer extensibility is taken into account which turns out to be essentially for the polymer conformations. Our analytical calculations predict a strong dependence of the relaxation times on the activity. In particular, semi- flexible polymers exhibit a crossover from a bending-elasticity-dominated to the flexible-polymer dynamics with increasing activity. This leads to a significant noise-induced polymer shrinkage over a large range of self-propulsion velocities. For large activities, the polymers swell and their extension becomes comparable to the contour length. The scaling properties of the mean square end-to-end distance with respect to the polymer length and monomer activity are discussed.
title Conformational properties of active semiflexible polymers
topic Soft Condensed Matter
url https://arxiv.org/abs/1610.07974