Large memcapacitance and memristance at Nb:SrTiO$_{3}$ / La$_{0.5}$Sr$_{0.5}$Mn$_{0.5}$Co$_{0.5}$O$_{3-δ}$ Topotactic Redox Interface

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Main Authors: Acevedo, W. R., Bosch, C. A. M. van den, Aguirre, M. H., Acha, C., Cavallaro, A., Ferreyra, C., Sánchez, M. J., Patrone, L., Aguadero, A., Rubi, D.
Format: Preprint
Published: 2019
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author Acevedo, W. R.
Bosch, C. A. M. van den
Aguirre, M. H.
Acha, C.
Cavallaro, A.
Ferreyra, C.
Sánchez, M. J.
Patrone, L.
Aguadero, A.
Rubi, D.
author_facet Acevedo, W. R.
Bosch, C. A. M. van den
Aguirre, M. H.
Acha, C.
Cavallaro, A.
Ferreyra, C.
Sánchez, M. J.
Patrone, L.
Aguadero, A.
Rubi, D.
contents The possibility to develop neuromorphic computing devices able to mimic the extraordinary data processing capabilities of biological systems spurs the research on memristive systems. Memristors with additional functionalities such as robust memcapacitance can outperform standard devices in key aspects such as power consumption or miniaturization possibilities. In this work, we demonstrate a large memcapacitive response of a perovskite memristive interface, using the topotactic redox ability of La$_{0.5}$Sr$_{0.5}$Mn$_{0.5}$Co$_{0.5}$O$_{3-δ}$ (LSMCO, 0 $\leq$ $δ$ $\leq$ 0.62). We demonstrate that the multi-mem behaviour originates at the switchable n-p diode formed at the Nb:SrTiO3/LSMCO interface. We found for our Nb:SrTiO$_{3}$/LSMCO/Pt devices a memcapacitive effect C$_{HIGH}$/C$_{LOW}$ ~ 100 at 150 kHz. The proof-of-concept interface reported here opens a promising venue to use topotactic redox materials for disruptive nanoelectronics, with straightforward applications in neuromorphic computing technology.
format Preprint
id arxiv_https___arxiv_org_abs_1905_05711
institution arXiv
publishDate 2019
record_format arxiv
spellingShingle Large memcapacitance and memristance at Nb:SrTiO$_{3}$ / La$_{0.5}$Sr$_{0.5}$Mn$_{0.5}$Co$_{0.5}$O$_{3-δ}$ Topotactic Redox Interface
Acevedo, W. R.
Bosch, C. A. M. van den
Aguirre, M. H.
Acha, C.
Cavallaro, A.
Ferreyra, C.
Sánchez, M. J.
Patrone, L.
Aguadero, A.
Rubi, D.
Applied Physics
Materials Science
The possibility to develop neuromorphic computing devices able to mimic the extraordinary data processing capabilities of biological systems spurs the research on memristive systems. Memristors with additional functionalities such as robust memcapacitance can outperform standard devices in key aspects such as power consumption or miniaturization possibilities. In this work, we demonstrate a large memcapacitive response of a perovskite memristive interface, using the topotactic redox ability of La$_{0.5}$Sr$_{0.5}$Mn$_{0.5}$Co$_{0.5}$O$_{3-δ}$ (LSMCO, 0 $\leq$ $δ$ $\leq$ 0.62). We demonstrate that the multi-mem behaviour originates at the switchable n-p diode formed at the Nb:SrTiO3/LSMCO interface. We found for our Nb:SrTiO$_{3}$/LSMCO/Pt devices a memcapacitive effect C$_{HIGH}$/C$_{LOW}$ ~ 100 at 150 kHz. The proof-of-concept interface reported here opens a promising venue to use topotactic redox materials for disruptive nanoelectronics, with straightforward applications in neuromorphic computing technology.
title Large memcapacitance and memristance at Nb:SrTiO$_{3}$ / La$_{0.5}$Sr$_{0.5}$Mn$_{0.5}$Co$_{0.5}$O$_{3-δ}$ Topotactic Redox Interface
topic Applied Physics
Materials Science
url https://arxiv.org/abs/1905.05711