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Main Authors: Zhang, Peng, Liu, Bo, Zhang, Shengli, Haule, K., Dai, Jianhui
Format: Preprint
Published: 2019
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Online Access:https://arxiv.org/abs/1909.13251
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author Zhang, Peng
Liu, Bo
Zhang, Shengli
Haule, K.
Dai, Jianhui
author_facet Zhang, Peng
Liu, Bo
Zhang, Shengli
Haule, K.
Dai, Jianhui
contents Nozi$\grave{e}$res' exhaustion theory argues the temperature for coherently screening of all local moments in Kondo lattice could be much lower than the temperature of single moment screening with insufficient number of conduction electrons. Recent experiment [Luo et al, PNAS, 112,13520 (2015)] indicates the cerium based nickel pnictides $CeNi_{2-δ}As_2 (δ\approx0.28)$ with low carrier density is an ideal material to exam such protracted Kondo screening. Using the density functional theory and dynamical mean-field theory, we calculated the respective electronic structures of paramagnetic $CeNi_2As_2$/$CeNi_2P_2$. In contrast to structurally analogous layered iron pnictides, the electronic structures of the present systems show strong three-dimensionality with substantially small contributions of Ni-3d electrons to the carrier density. Moreover, we find significant Kondo resonance peaks in the compressed $CeNi_2As_2$ and $CeNi_2P_2$ at low temperatures, accompanied by topological changes of the Fermi surfaces. We also find similar quantum phase transition in $CeNi_2As_2$ driven by chemical pressure via the isovalence As$\rightarrow$P substitution.
format Preprint
id arxiv_https___arxiv_org_abs_1909_13251
institution arXiv
publishDate 2019
record_format arxiv
spellingShingle Protracted Kondo coherence with dilute carrier density in Cerium based nickel pnictides
Zhang, Peng
Liu, Bo
Zhang, Shengli
Haule, K.
Dai, Jianhui
Strongly Correlated Electrons
Nozi$\grave{e}$res' exhaustion theory argues the temperature for coherently screening of all local moments in Kondo lattice could be much lower than the temperature of single moment screening with insufficient number of conduction electrons. Recent experiment [Luo et al, PNAS, 112,13520 (2015)] indicates the cerium based nickel pnictides $CeNi_{2-δ}As_2 (δ\approx0.28)$ with low carrier density is an ideal material to exam such protracted Kondo screening. Using the density functional theory and dynamical mean-field theory, we calculated the respective electronic structures of paramagnetic $CeNi_2As_2$/$CeNi_2P_2$. In contrast to structurally analogous layered iron pnictides, the electronic structures of the present systems show strong three-dimensionality with substantially small contributions of Ni-3d electrons to the carrier density. Moreover, we find significant Kondo resonance peaks in the compressed $CeNi_2As_2$ and $CeNi_2P_2$ at low temperatures, accompanied by topological changes of the Fermi surfaces. We also find similar quantum phase transition in $CeNi_2As_2$ driven by chemical pressure via the isovalence As$\rightarrow$P substitution.
title Protracted Kondo coherence with dilute carrier density in Cerium based nickel pnictides
topic Strongly Correlated Electrons
url https://arxiv.org/abs/1909.13251