Generation of even and odd high harmonics in resonant metasurfaces using single and multiple ultra-intense laser pulses

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Main Authors: Shcherbakov, Maxim R., Zhang, Haizhong, Tripepi, Michael, Sartorello, Giovanni, Talisa, Noah, AlShafey, Abdallah, Fan, Zhiyuan, Twardowski, Justin, Krivitsky, Leonid A., Kuznetsov, Arseniy I., Chowdhury, Enam, Shvets, Gennady
Format: Preprint
Published: 2020
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author Shcherbakov, Maxim R.
Zhang, Haizhong
Tripepi, Michael
Sartorello, Giovanni
Talisa, Noah
AlShafey, Abdallah
Fan, Zhiyuan
Twardowski, Justin
Krivitsky, Leonid A.
Kuznetsov, Arseniy I.
Chowdhury, Enam
Shvets, Gennady
author_facet Shcherbakov, Maxim R.
Zhang, Haizhong
Tripepi, Michael
Sartorello, Giovanni
Talisa, Noah
AlShafey, Abdallah
Fan, Zhiyuan
Twardowski, Justin
Krivitsky, Leonid A.
Kuznetsov, Arseniy I.
Chowdhury, Enam
Shvets, Gennady
contents High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in nanostructures is an attractive route to overcoming the well-known limitations of gases and bulk solids. We demonstrate a nanoscale platform for highly efficient HHG driven by strong mid-infrared laser pulses: an ultra-thin resonant gallium phosphide (GaP) metasurface. The wide bandgap and the lack of inversion symmetry of the GaP crystal enable the generation of even and odd harmonics covering a wide range of photon energies between 1.3 and 3 eV with minimal reabsorption. The resonantly enhanced conversion efficiency facilitates single-shot measurements that avoid material damage and pave the way to controllable transition between perturbative and non-perturbative regimes of light-matter interactions at the nanoscale.
format Preprint
id arxiv_https___arxiv_org_abs_2008_03619
institution arXiv
publishDate 2020
record_format arxiv
spellingShingle Generation of even and odd high harmonics in resonant metasurfaces using single and multiple ultra-intense laser pulses
Shcherbakov, Maxim R.
Zhang, Haizhong
Tripepi, Michael
Sartorello, Giovanni
Talisa, Noah
AlShafey, Abdallah
Fan, Zhiyuan
Twardowski, Justin
Krivitsky, Leonid A.
Kuznetsov, Arseniy I.
Chowdhury, Enam
Shvets, Gennady
Optics
Mesoscale and Nanoscale Physics
High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in nanostructures is an attractive route to overcoming the well-known limitations of gases and bulk solids. We demonstrate a nanoscale platform for highly efficient HHG driven by strong mid-infrared laser pulses: an ultra-thin resonant gallium phosphide (GaP) metasurface. The wide bandgap and the lack of inversion symmetry of the GaP crystal enable the generation of even and odd harmonics covering a wide range of photon energies between 1.3 and 3 eV with minimal reabsorption. The resonantly enhanced conversion efficiency facilitates single-shot measurements that avoid material damage and pave the way to controllable transition between perturbative and non-perturbative regimes of light-matter interactions at the nanoscale.
title Generation of even and odd high harmonics in resonant metasurfaces using single and multiple ultra-intense laser pulses
topic Optics
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2008.03619