a-axis YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x trilayers with subnanometer rms roughness

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Auteurs principaux: Suyolcu, Y. Eren, Sun, Jiaxin, Goodge, Berit H., Park, Jisung, Schubert, Jürgen, Kourkoutis, Lena F., Schlom, Darrell G.
Format: Preprint
Publié: 2020
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author Suyolcu, Y. Eren
Sun, Jiaxin
Goodge, Berit H.
Park, Jisung
Schubert, Jürgen
Kourkoutis, Lena F.
Schlom, Darrell G.
author_facet Suyolcu, Y. Eren
Sun, Jiaxin
Goodge, Berit H.
Park, Jisung
Schubert, Jürgen
Kourkoutis, Lena F.
Schlom, Darrell G.
contents We demonstrate a-axis YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x trilayers grown on (100) LaAlO3 substrates with improved interface smoothness. The trilayers are synthesized by ozone-assisted molecular-beam epitaxy. The thickness of the PrBa2Cu3O7-x layer is held constant at 8 nm and the thickness of the YBa2Cu3O7-x layers is varied from 24 nm to 100 nm. X-ray diffraction measurements show all trilayers to have >95% a-axis content. The rms roughness of the thinnest trilayer is < 0.7 nm and this roughness increases with the thickness of the YBa2Cu3O7-x layers. The thickness of the YBa2Cu3O7-x layers also affects the transport properties: while all samples exhibit an onset of the superconducting transition at and above 85 K, the thinner samples show wider transition widths, ΔTc. High-resolution scanning transmission electron microscopy reveals coherent and chemically sharp interfaces, and that growth begins with a cubic (Y,Ba)CuO3-x perovskite phase that transforms into a-axis oriented YBa2Cu3O7-x as the substrate temperature is ramped up.
format Preprint
id arxiv_https___arxiv_org_abs_2010_12624
institution arXiv
publishDate 2020
record_format arxiv
spellingShingle a-axis YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x trilayers with subnanometer rms roughness
Suyolcu, Y. Eren
Sun, Jiaxin
Goodge, Berit H.
Park, Jisung
Schubert, Jürgen
Kourkoutis, Lena F.
Schlom, Darrell G.
Superconductivity
Materials Science
We demonstrate a-axis YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x trilayers grown on (100) LaAlO3 substrates with improved interface smoothness. The trilayers are synthesized by ozone-assisted molecular-beam epitaxy. The thickness of the PrBa2Cu3O7-x layer is held constant at 8 nm and the thickness of the YBa2Cu3O7-x layers is varied from 24 nm to 100 nm. X-ray diffraction measurements show all trilayers to have >95% a-axis content. The rms roughness of the thinnest trilayer is < 0.7 nm and this roughness increases with the thickness of the YBa2Cu3O7-x layers. The thickness of the YBa2Cu3O7-x layers also affects the transport properties: while all samples exhibit an onset of the superconducting transition at and above 85 K, the thinner samples show wider transition widths, ΔTc. High-resolution scanning transmission electron microscopy reveals coherent and chemically sharp interfaces, and that growth begins with a cubic (Y,Ba)CuO3-x perovskite phase that transforms into a-axis oriented YBa2Cu3O7-x as the substrate temperature is ramped up.
title a-axis YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x trilayers with subnanometer rms roughness
topic Superconductivity
Materials Science
url https://arxiv.org/abs/2010.12624