New Experimentally Observable Gamma-ray Emissions from 241Am Nuclear Decay

Fuente: arXiv
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Hauptverfasser: Koehler, Katrina E., Yoho, Michael D., Carpenter, Matthew H., Croce, Mark P., Mercer, David J., Smith, Chandler M., Tollefson, Aidan D., Vo, Duc T., Famiano, Michael A., Nesaraja, Caroline D., Becker, Daniel T., Gard, Johnathon D., Wessels, Abigail L., Bennett, Douglas A., Mates, J. A. B., Ortiz, Nathan J., Schmidt, Daniel R., Ullom, Joel N., Vale, Leila R.
Format: Preprint
Veröffentlicht: 2021
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author Koehler, Katrina E.
Yoho, Michael D.
Carpenter, Matthew H.
Croce, Mark P.
Mercer, David J.
Smith, Chandler M.
Tollefson, Aidan D.
Vo, Duc T.
Famiano, Michael A.
Nesaraja, Caroline D.
Becker, Daniel T.
Gard, Johnathon D.
Wessels, Abigail L.
Bennett, Douglas A.
Mates, J. A. B.
Ortiz, Nathan J.
Schmidt, Daniel R.
Ullom, Joel N.
Vale, Leila R.
author_facet Koehler, Katrina E.
Yoho, Michael D.
Carpenter, Matthew H.
Croce, Mark P.
Mercer, David J.
Smith, Chandler M.
Tollefson, Aidan D.
Vo, Duc T.
Famiano, Michael A.
Nesaraja, Caroline D.
Becker, Daniel T.
Gard, Johnathon D.
Wessels, Abigail L.
Bennett, Douglas A.
Mates, J. A. B.
Ortiz, Nathan J.
Schmidt, Daniel R.
Ullom, Joel N.
Vale, Leila R.
contents With the high resolution of microcalorimeter detectors, previously unresolvable gamma-ray lines are now clearly resolvable. A careful measurement of Am-241 decay with a large array of gamma-ray microcalorimeters has revealed never before seen or predicted gamma lines at 207.72 +/- 0.02 keV and 208.21 +/- 0.01 keV. These results were made possible by new microwave-multiplexing readout to increase the array size and improved analysis algorithms to eliminate spectral artifacts. We suggest nuclear levels from which these gamma-rays might originate and calculate branching ratios for these transitions from measurements of both mixed Pu-Am standards and a pure Am-241 source. These results have implications for nuclear material safeguards and accounting, particularly for microcalorimeter gamma spectrometers, which are now being adopted in nuclear safeguards analytical laboratories.
format Preprint
id arxiv_https___arxiv_org_abs_2103_15893
institution arXiv
publishDate 2021
record_format arxiv
spellingShingle New Experimentally Observable Gamma-ray Emissions from 241Am Nuclear Decay
Koehler, Katrina E.
Yoho, Michael D.
Carpenter, Matthew H.
Croce, Mark P.
Mercer, David J.
Smith, Chandler M.
Tollefson, Aidan D.
Vo, Duc T.
Famiano, Michael A.
Nesaraja, Caroline D.
Becker, Daniel T.
Gard, Johnathon D.
Wessels, Abigail L.
Bennett, Douglas A.
Mates, J. A. B.
Ortiz, Nathan J.
Schmidt, Daniel R.
Ullom, Joel N.
Vale, Leila R.
Nuclear Experiment
With the high resolution of microcalorimeter detectors, previously unresolvable gamma-ray lines are now clearly resolvable. A careful measurement of Am-241 decay with a large array of gamma-ray microcalorimeters has revealed never before seen or predicted gamma lines at 207.72 +/- 0.02 keV and 208.21 +/- 0.01 keV. These results were made possible by new microwave-multiplexing readout to increase the array size and improved analysis algorithms to eliminate spectral artifacts. We suggest nuclear levels from which these gamma-rays might originate and calculate branching ratios for these transitions from measurements of both mixed Pu-Am standards and a pure Am-241 source. These results have implications for nuclear material safeguards and accounting, particularly for microcalorimeter gamma spectrometers, which are now being adopted in nuclear safeguards analytical laboratories.
title New Experimentally Observable Gamma-ray Emissions from 241Am Nuclear Decay
topic Nuclear Experiment
url https://arxiv.org/abs/2103.15893