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Main Authors: Bhowal, Sayantika, O'Neill, Daniel, Fechner, Michael, Spaldin, Nicola A., Staub, Urs, Duffy, Jon, Collins, Stephen P.
Format: Preprint
Published: 2021
Subjects:
Online Access:https://arxiv.org/abs/2106.02431
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author Bhowal, Sayantika
O'Neill, Daniel
Fechner, Michael
Spaldin, Nicola A.
Staub, Urs
Duffy, Jon
Collins, Stephen P.
author_facet Bhowal, Sayantika
O'Neill, Daniel
Fechner, Michael
Spaldin, Nicola A.
Staub, Urs
Duffy, Jon
Collins, Stephen P.
contents We present a combined theoretical and experimental investigation of the anti-symmetric Compton profile in LiNiPO$_4$ as a possible probe for magneto-electric toroidal moments. Understanding as well as detecting such magneto-electric multipoles is an active area of research in condensed matter physics. Our calculations, based on density functional theory, indicate an anti-symmetric Compton profile in the direction of the $t_y$ toroidal moment in momentum space, with the computed anti-symmetric profile around four orders of magnitude smaller than the total profile. The difference signal that we measure is consistent with the computed profile, but of the same order of magnitude as the statistical errors and systematic uncertainties of the experiment. Our results motivate further theoretical work to understand the factors that influence the size of the anti-symmetric Compton profile, and to identify materials exhibiting larger effects.
format Preprint
id arxiv_https___arxiv_org_abs_2106_02431
institution arXiv
publishDate 2021
record_format arxiv
spellingShingle Anti-symmetric Compton scattering in LiNiPO$_4$: Towards a direct probe of the magneto-electric multipole moment
Bhowal, Sayantika
O'Neill, Daniel
Fechner, Michael
Spaldin, Nicola A.
Staub, Urs
Duffy, Jon
Collins, Stephen P.
Materials Science
We present a combined theoretical and experimental investigation of the anti-symmetric Compton profile in LiNiPO$_4$ as a possible probe for magneto-electric toroidal moments. Understanding as well as detecting such magneto-electric multipoles is an active area of research in condensed matter physics. Our calculations, based on density functional theory, indicate an anti-symmetric Compton profile in the direction of the $t_y$ toroidal moment in momentum space, with the computed anti-symmetric profile around four orders of magnitude smaller than the total profile. The difference signal that we measure is consistent with the computed profile, but of the same order of magnitude as the statistical errors and systematic uncertainties of the experiment. Our results motivate further theoretical work to understand the factors that influence the size of the anti-symmetric Compton profile, and to identify materials exhibiting larger effects.
title Anti-symmetric Compton scattering in LiNiPO$_4$: Towards a direct probe of the magneto-electric multipole moment
topic Materials Science
url https://arxiv.org/abs/2106.02431