Understanding the nonlinear optical response of epsilon near zero materials in the time-domain

Fuente: arXiv
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Autori principali: Baxter, Joshua, Pérez-Casanova, Adriana, Cortes-Herrera, Luis, Lesina, Antonio Calà, De Leon, Israel, Ramunno, Lora
Natura: Preprint
Pubblicazione: 2021
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author Baxter, Joshua
Pérez-Casanova, Adriana
Cortes-Herrera, Luis
Lesina, Antonio Calà
De Leon, Israel
Ramunno, Lora
author_facet Baxter, Joshua
Pérez-Casanova, Adriana
Cortes-Herrera, Luis
Lesina, Antonio Calà
De Leon, Israel
Ramunno, Lora
contents The promise of active nanophotonics technology relies on the confinement and control of light at the nanoscale. Confinement via plasmonics, dielectric resonators, and waveguides can be complemented with materials whose optical properties can be controlled using nonlinear effects. Transparent conducting oxides (TCOs) exhibit strong optical nonlinearities in their near zero permittivity spectral region, on the femtosecond time-scale. Harnessing full control over the nonlinear response requires a deeper understanding of the process. To achieve this, we develop a self-consistent time-domain model for the nonlinear optical response of TCOs and implement it into a three-dimensional finite-difference time-domain code. We compare and tune our simulation tools against recently published experimental results for intense laser irradiation of thin indium tin oxide (ITO) films. Finally, by simulating intense laser irradiation of ITO-based plasmonic metasurfaces, we demonstrate the full power of our approach. As expected, we find validating the significant enhancement of the nonlinear response of an ITO-based metasurface over bare ITO thin films. Our work thus enables quantitative nanophotonics design with epsilon-near-zero materials.
format Preprint
id arxiv_https___arxiv_org_abs_2110_14806
institution arXiv
publishDate 2021
record_format arxiv
spellingShingle Understanding the nonlinear optical response of epsilon near zero materials in the time-domain
Baxter, Joshua
Pérez-Casanova, Adriana
Cortes-Herrera, Luis
Lesina, Antonio Calà
De Leon, Israel
Ramunno, Lora
Optics
Computational Physics
The promise of active nanophotonics technology relies on the confinement and control of light at the nanoscale. Confinement via plasmonics, dielectric resonators, and waveguides can be complemented with materials whose optical properties can be controlled using nonlinear effects. Transparent conducting oxides (TCOs) exhibit strong optical nonlinearities in their near zero permittivity spectral region, on the femtosecond time-scale. Harnessing full control over the nonlinear response requires a deeper understanding of the process. To achieve this, we develop a self-consistent time-domain model for the nonlinear optical response of TCOs and implement it into a three-dimensional finite-difference time-domain code. We compare and tune our simulation tools against recently published experimental results for intense laser irradiation of thin indium tin oxide (ITO) films. Finally, by simulating intense laser irradiation of ITO-based plasmonic metasurfaces, we demonstrate the full power of our approach. As expected, we find validating the significant enhancement of the nonlinear response of an ITO-based metasurface over bare ITO thin films. Our work thus enables quantitative nanophotonics design with epsilon-near-zero materials.
title Understanding the nonlinear optical response of epsilon near zero materials in the time-domain
topic Optics
Computational Physics
url https://arxiv.org/abs/2110.14806