Charge-4e and charge-6e flux quantization and higher charge superconductivity in kagome superconductor ring devices

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Hauptverfasser: Ge, Jun, Wang, Pinyuan, Xing, Ying, Yin, Qiangwei, Wang, Anqi, Shen, Jie, Lei, Hechang, Wang, Ziqiang, Wang, Jian
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Veröffentlicht: 2022
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author Ge, Jun
Wang, Pinyuan
Xing, Ying
Yin, Qiangwei
Wang, Anqi
Shen, Jie
Lei, Hechang
Wang, Ziqiang
Wang, Jian
author_facet Ge, Jun
Wang, Pinyuan
Xing, Ying
Yin, Qiangwei
Wang, Anqi
Shen, Jie
Lei, Hechang
Wang, Ziqiang
Wang, Jian
contents The flux quantization is a key indication of electron pairing in superconductors. For example, the well-known h/2e flux quantization is considered strong evidence for the existence of the charge-2e, two-electron Cooper pairs. Here we report evidence for multi-charge flux quantization in mesoscopic ring devices fabricated using the transition-metal kagome superconductor CsV3Sb5. We perform systematic magneto-transport measurements and observe unprecedented quantization of magnetic flux in units of h/4e and h/6e in magnetoresistance oscillations. Specifically, at low temperatures, magnetoresistance oscillations with period h/2e are detected, as expected from the flux quantization for charge-2e superconductivity. We find that the h/2e oscillations are suppressed and replaced by resistance oscillations with h/4e periodicity when temperature is increased. Increasing the temperature further suppresses the h/4e oscillations and robust resistance oscillations with h/6e periodicity emerge as evidence for charge-6e flux quantization. Our observations provide the first experimental evidence for the existence of multi-charge flux quanta and emergent quantum matter exhibiting higher-charge superconductivity in the strongly fluctuating region above the charge-2e Cooper pair condensate, revealing new insights into the intertwined and vestigial electronic order in kagome superconductors.
format Preprint
id arxiv_https___arxiv_org_abs_2201_10352
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Charge-4e and charge-6e flux quantization and higher charge superconductivity in kagome superconductor ring devices
Ge, Jun
Wang, Pinyuan
Xing, Ying
Yin, Qiangwei
Wang, Anqi
Shen, Jie
Lei, Hechang
Wang, Ziqiang
Wang, Jian
Superconductivity
Mesoscale and Nanoscale Physics
Materials Science
The flux quantization is a key indication of electron pairing in superconductors. For example, the well-known h/2e flux quantization is considered strong evidence for the existence of the charge-2e, two-electron Cooper pairs. Here we report evidence for multi-charge flux quantization in mesoscopic ring devices fabricated using the transition-metal kagome superconductor CsV3Sb5. We perform systematic magneto-transport measurements and observe unprecedented quantization of magnetic flux in units of h/4e and h/6e in magnetoresistance oscillations. Specifically, at low temperatures, magnetoresistance oscillations with period h/2e are detected, as expected from the flux quantization for charge-2e superconductivity. We find that the h/2e oscillations are suppressed and replaced by resistance oscillations with h/4e periodicity when temperature is increased. Increasing the temperature further suppresses the h/4e oscillations and robust resistance oscillations with h/6e periodicity emerge as evidence for charge-6e flux quantization. Our observations provide the first experimental evidence for the existence of multi-charge flux quanta and emergent quantum matter exhibiting higher-charge superconductivity in the strongly fluctuating region above the charge-2e Cooper pair condensate, revealing new insights into the intertwined and vestigial electronic order in kagome superconductors.
title Charge-4e and charge-6e flux quantization and higher charge superconductivity in kagome superconductor ring devices
topic Superconductivity
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2201.10352