Pressure-induced reemergence of superconductivity in BaIr2Ge7 and Ba3Ir4Ge16 with cage structures

Fuente: arXiv
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Autori principali: Pei, Cuiying, Ying, Tianping, Zhao, Yi, Gao, Lingling, Cao, Weizheng, Li, Changhua, Hosono, Hideo, Qi, Yanpeng
Natura: Preprint
Pubblicazione: 2022
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author Pei, Cuiying
Ying, Tianping
Zhao, Yi
Gao, Lingling
Cao, Weizheng
Li, Changhua
Hosono, Hideo
Qi, Yanpeng
author_facet Pei, Cuiying
Ying, Tianping
Zhao, Yi
Gao, Lingling
Cao, Weizheng
Li, Changhua
Hosono, Hideo
Qi, Yanpeng
contents The clathrate-like or caged compounds have attracted continuing interest due to their structural flexibility as well as fertile physical properties. Here we report a pressure-induced reemergence of superconductivity in BaIr2Ge7 and Ba3Ir4Ge16, two new caged superconductors with two-dimensional building blocks of cage structures. After suppressing the ambient-pressure superconducting (SC-I) state, a new superconducting (SC-II) state emerges unexpectedly, with Tc increased to a maximum of 4.4 K and 4.0 K for BaIr2Ge7 and Ba3Ir4Ge16, respectively. Combined with high-pressure synchrotron x-ray diffraction and Raman measurements, we propose that the reemergence of superconductivity in the caged superconductors can be ascribed to a pressure-induced phonon softening linked to the cage shrink.
format Preprint
id arxiv_https___arxiv_org_abs_2202_04493
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Pressure-induced reemergence of superconductivity in BaIr2Ge7 and Ba3Ir4Ge16 with cage structures
Pei, Cuiying
Ying, Tianping
Zhao, Yi
Gao, Lingling
Cao, Weizheng
Li, Changhua
Hosono, Hideo
Qi, Yanpeng
Superconductivity
Materials Science
The clathrate-like or caged compounds have attracted continuing interest due to their structural flexibility as well as fertile physical properties. Here we report a pressure-induced reemergence of superconductivity in BaIr2Ge7 and Ba3Ir4Ge16, two new caged superconductors with two-dimensional building blocks of cage structures. After suppressing the ambient-pressure superconducting (SC-I) state, a new superconducting (SC-II) state emerges unexpectedly, with Tc increased to a maximum of 4.4 K and 4.0 K for BaIr2Ge7 and Ba3Ir4Ge16, respectively. Combined with high-pressure synchrotron x-ray diffraction and Raman measurements, we propose that the reemergence of superconductivity in the caged superconductors can be ascribed to a pressure-induced phonon softening linked to the cage shrink.
title Pressure-induced reemergence of superconductivity in BaIr2Ge7 and Ba3Ir4Ge16 with cage structures
topic Superconductivity
Materials Science
url https://arxiv.org/abs/2202.04493