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Auteurs principaux: Peng, Wei, Park, Se Young, Roh, Chang Jae, Mun, Junsik, Ju, Hwiin, Kim, Jinkwon, Ko, Eun Kyo, Liang, Zhengguo, Hahn, Sungsoo, Zhang, Jinfeng, Si, Liang, Jo, Yong Jin, Kim, Tae Heon, Kim, Changyoung, Wang, Lingfei, Kim, Miyoung, Lee, Jong Seok, Noh, Tae Won, Lee, Daesu
Format: Preprint
Publié: 2022
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Accès en ligne:https://arxiv.org/abs/2203.03199
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author Peng, Wei
Park, Se Young
Roh, Chang Jae
Mun, Junsik
Ju, Hwiin
Kim, Jinkwon
Ko, Eun Kyo
Liang, Zhengguo
Hahn, Sungsoo
Zhang, Jinfeng
Si, Liang
Jo, Yong Jin
Kim, Tae Heon
Kim, Changyoung
Wang, Lingfei
Kim, Miyoung
Lee, Jong Seok
Noh, Tae Won
Lee, Daesu
author_facet Peng, Wei
Park, Se Young
Roh, Chang Jae
Mun, Junsik
Ju, Hwiin
Kim, Jinkwon
Ko, Eun Kyo
Liang, Zhengguo
Hahn, Sungsoo
Zhang, Jinfeng
Si, Liang
Jo, Yong Jin
Kim, Tae Heon
Kim, Changyoung
Wang, Lingfei
Kim, Miyoung
Lee, Jong Seok
Noh, Tae Won
Lee, Daesu
contents Electric fields have played a key role in discovering and controlling exotic electronic states of condensed matter. However, electric fields usually do not work in metals as free carriers tend to screen electrostatic fields. While a pseudo-electric field generated by inhomogeneous lattice strain, namely a flexoelectric field, can in principle work in all classes of materials, it remains experimentally unexplored in metals. Here, using heteroepitaxy and atomic-scale imaging, we show that flexoelectric fields can polarize a metallic oxide SrRuO3 with unexpectedly large Ru off-center displacements. We also observe that the flexoelectrically induced polar state of SrRuO3 leads to sizable lattice expansion, similar to the electrostrictive expansion caused by ionic displacements in dielectrics under an external electric field. We further suggest that flexoelectrically driven Ru off-centering promotes strong coupling between lattice and electronic degrees of freedom, possibly enhancing the ferromagnetism of SrRuO3. Beyond conventional electric fields, flexoelectric fields may universally engender novel electronic states and their control via pure atomic displacements in a nondestructive and fast manner.
format Preprint
id arxiv_https___arxiv_org_abs_2203_03199
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Flexoelectric control of a ferromagnetic metal
Peng, Wei
Park, Se Young
Roh, Chang Jae
Mun, Junsik
Ju, Hwiin
Kim, Jinkwon
Ko, Eun Kyo
Liang, Zhengguo
Hahn, Sungsoo
Zhang, Jinfeng
Si, Liang
Jo, Yong Jin
Kim, Tae Heon
Kim, Changyoung
Wang, Lingfei
Kim, Miyoung
Lee, Jong Seok
Noh, Tae Won
Lee, Daesu
Materials Science
Strongly Correlated Electrons
Electric fields have played a key role in discovering and controlling exotic electronic states of condensed matter. However, electric fields usually do not work in metals as free carriers tend to screen electrostatic fields. While a pseudo-electric field generated by inhomogeneous lattice strain, namely a flexoelectric field, can in principle work in all classes of materials, it remains experimentally unexplored in metals. Here, using heteroepitaxy and atomic-scale imaging, we show that flexoelectric fields can polarize a metallic oxide SrRuO3 with unexpectedly large Ru off-center displacements. We also observe that the flexoelectrically induced polar state of SrRuO3 leads to sizable lattice expansion, similar to the electrostrictive expansion caused by ionic displacements in dielectrics under an external electric field. We further suggest that flexoelectrically driven Ru off-centering promotes strong coupling between lattice and electronic degrees of freedom, possibly enhancing the ferromagnetism of SrRuO3. Beyond conventional electric fields, flexoelectric fields may universally engender novel electronic states and their control via pure atomic displacements in a nondestructive and fast manner.
title Flexoelectric control of a ferromagnetic metal
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2203.03199