Scattering-asymmetry control with ultrafast electron wave packet shaping

Fuente: arXiv
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Autori principali: Morimoto, Yuya, Hommelhoff, Peter, Madsen, Lars Bojer
Natura: Preprint
Pubblicazione: 2022
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author Morimoto, Yuya
Hommelhoff, Peter
Madsen, Lars Bojer
author_facet Morimoto, Yuya
Hommelhoff, Peter
Madsen, Lars Bojer
contents Scattering of a tightly focused electron beam by an atom forms one of the bases of modern electron microscopy. A fundamental symmetry breaking occurs when the target atom is displaced from the beam center. This displacement results in a deflection of the beam and an asymmetric angular distribution of the scattered electrons. Here we propose a concept to control the sign and magnitude of the scattering asymmetry by shaping the incident high-energy electron wave packet in momentum space on the atto- to picosecond time scale. The shaping controls the ultrafast real-space dynamics of the wave packet, shifting the balance between two competing contributions of the impact-parameter-dependent quantum interference and the momentum distribution of the wave packet on the target. We find a strong sensitivity of the elastic scattering on the wave packet properties, an effect that will allow wave-packet and target characterization in ultrafast electron microscopy.
format Preprint
id arxiv_https___arxiv_org_abs_2203_13425
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Scattering-asymmetry control with ultrafast electron wave packet shaping
Morimoto, Yuya
Hommelhoff, Peter
Madsen, Lars Bojer
Atomic Physics
Scattering of a tightly focused electron beam by an atom forms one of the bases of modern electron microscopy. A fundamental symmetry breaking occurs when the target atom is displaced from the beam center. This displacement results in a deflection of the beam and an asymmetric angular distribution of the scattered electrons. Here we propose a concept to control the sign and magnitude of the scattering asymmetry by shaping the incident high-energy electron wave packet in momentum space on the atto- to picosecond time scale. The shaping controls the ultrafast real-space dynamics of the wave packet, shifting the balance between two competing contributions of the impact-parameter-dependent quantum interference and the momentum distribution of the wave packet on the target. We find a strong sensitivity of the elastic scattering on the wave packet properties, an effect that will allow wave-packet and target characterization in ultrafast electron microscopy.
title Scattering-asymmetry control with ultrafast electron wave packet shaping
topic Atomic Physics
url https://arxiv.org/abs/2203.13425