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Auteurs principaux: Maluski, D., Mayorga, I. Cámara, Hemberger, J., Grüninger, M.
Format: Preprint
Publié: 2022
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Accès en ligne:https://arxiv.org/abs/2203.13660
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author Maluski, D.
Mayorga, I. Cámara
Hemberger, J.
Grüninger, M.
author_facet Maluski, D.
Mayorga, I. Cámara
Hemberger, J.
Grüninger, M.
contents For terahertz spectroscopy on single crystals, the wavelength $λ$ often is comparable to the size of the studied samples, emphasizing diffraction effects. Using a continuous-wave terahertz spectrometer in transmission geometry, we address the effect of the sample size on the achievable accuracy of the optical properties, focusing in particular on the phase data. We employ $α$-lactose monohydrate as a paradigmatic example and compare data that were measured using apertures with diameters D in the range from 10 mm to 0.2 mm. For small D, strong diffraction typically invalidates a quantitative analysis of the transmitted amplitude at low frequencies. The phase data, however, can be evaluated to lower frequency and show a more systematic dependence on D. For a quantitative analysis, we employ a waveguide picture for the description of small apertures with a cylindrical bore. For D as small as 0.2 mm, corresponding to 1/D = 50 cm$^{-1}$, a circular waveguide does not support propagating waves below its cut-off frequency $1/λ_c = ω_c/2πc \approx 29$ cm$^{-1}$. Experimentally, we confirm this cut-off for cylindrical apertures with a thickness $d_{ap} = 1$ mm. Close to $ω_c$, the measured phase velocity is an order of magnitude larger than $c$, the speed of light in vacuum. The cut-off is washed out if a sample is mounted on a thin aperture with a conical bore. In this case, the phase data of $α$-lactose monohydrate for D = 0.2 mm can quantitatively be described down to about 10 cm$^{-1}$ if the waveguide-like properties of the aperture are taken into account in the analysis.
format Preprint
id arxiv_https___arxiv_org_abs_2203_13660
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Terahertz measurements on subwavelength-size samples down to the tunneling limit
Maluski, D.
Mayorga, I. Cámara
Hemberger, J.
Grüninger, M.
Optics
For terahertz spectroscopy on single crystals, the wavelength $λ$ often is comparable to the size of the studied samples, emphasizing diffraction effects. Using a continuous-wave terahertz spectrometer in transmission geometry, we address the effect of the sample size on the achievable accuracy of the optical properties, focusing in particular on the phase data. We employ $α$-lactose monohydrate as a paradigmatic example and compare data that were measured using apertures with diameters D in the range from 10 mm to 0.2 mm. For small D, strong diffraction typically invalidates a quantitative analysis of the transmitted amplitude at low frequencies. The phase data, however, can be evaluated to lower frequency and show a more systematic dependence on D. For a quantitative analysis, we employ a waveguide picture for the description of small apertures with a cylindrical bore. For D as small as 0.2 mm, corresponding to 1/D = 50 cm$^{-1}$, a circular waveguide does not support propagating waves below its cut-off frequency $1/λ_c = ω_c/2πc \approx 29$ cm$^{-1}$. Experimentally, we confirm this cut-off for cylindrical apertures with a thickness $d_{ap} = 1$ mm. Close to $ω_c$, the measured phase velocity is an order of magnitude larger than $c$, the speed of light in vacuum. The cut-off is washed out if a sample is mounted on a thin aperture with a conical bore. In this case, the phase data of $α$-lactose monohydrate for D = 0.2 mm can quantitatively be described down to about 10 cm$^{-1}$ if the waveguide-like properties of the aperture are taken into account in the analysis.
title Terahertz measurements on subwavelength-size samples down to the tunneling limit
topic Optics
url https://arxiv.org/abs/2203.13660