Neutral Silicon Vacancy Centers in Diamond via Photoactivated Itinerant Carriers

Fuente: arXiv
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Main Authors: Zhang, Zi-Huai, Edmonds, Andrew M., Palmer, Nicola, Markham, Matthew L., de Leon, Nathalie P.
Format: Preprint
Published: 2022
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author Zhang, Zi-Huai
Edmonds, Andrew M.
Palmer, Nicola
Markham, Matthew L.
de Leon, Nathalie P.
author_facet Zhang, Zi-Huai
Edmonds, Andrew M.
Palmer, Nicola
Markham, Matthew L.
de Leon, Nathalie P.
contents Neutral silicon vacancy (SiV0) centers in diamond are promising candidates for quantum network applications because of their exceptional optical properties and spin coherence. However, the stabilization of SiV0 centers requires careful Fermi level engineering of the diamond host material, making further technological development challenging. Here, we show that SiV0 centers can be efficiently stabilized by photoactivated itinerant carriers. Even in this nonequilibrium configuration, the resulting SiV0 centers are stable enough to allow for resonant optical excitation and optically detected magnetic resonance. Our results pave the way for on-demand generation of SiV0 centers as well as other emerging quantum defects in diamond.
format Preprint
id arxiv_https___arxiv_org_abs_2209_08710
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Neutral Silicon Vacancy Centers in Diamond via Photoactivated Itinerant Carriers
Zhang, Zi-Huai
Edmonds, Andrew M.
Palmer, Nicola
Markham, Matthew L.
de Leon, Nathalie P.
Quantum Physics
Materials Science
Neutral silicon vacancy (SiV0) centers in diamond are promising candidates for quantum network applications because of their exceptional optical properties and spin coherence. However, the stabilization of SiV0 centers requires careful Fermi level engineering of the diamond host material, making further technological development challenging. Here, we show that SiV0 centers can be efficiently stabilized by photoactivated itinerant carriers. Even in this nonequilibrium configuration, the resulting SiV0 centers are stable enough to allow for resonant optical excitation and optically detected magnetic resonance. Our results pave the way for on-demand generation of SiV0 centers as well as other emerging quantum defects in diamond.
title Neutral Silicon Vacancy Centers in Diamond via Photoactivated Itinerant Carriers
topic Quantum Physics
Materials Science
url https://arxiv.org/abs/2209.08710