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Main Authors: Luckin, W. R. B., Li, Y., Jiang, J., Gunasekera, S. M., Wen, C., Zhang, Y., Prabhakaran, D., Flicker, F., Chen, Y., Mucha-Kruczynski, M.
Format: Preprint
Published: 2022
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Online Access:https://arxiv.org/abs/2211.01780
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author Luckin, W. R. B.
Li, Y.
Jiang, J.
Gunasekera, S. M.
Wen, C.
Zhang, Y.
Prabhakaran, D.
Flicker, F.
Chen, Y.
Mucha-Kruczynski, M.
author_facet Luckin, W. R. B.
Li, Y.
Jiang, J.
Gunasekera, S. M.
Wen, C.
Zhang, Y.
Prabhakaran, D.
Flicker, F.
Chen, Y.
Mucha-Kruczynski, M.
contents We report on the interplay between a van Hove singularity and a charge density wave state in 2H-TaSe$_{2}$. We use angle-resolved photoemission spectroscopy to investigate changes in the Fermi surface of this material under surface doping with potassium. At high doping, we observe modifications which imply the disappearance of the $(3\times 3)$ charge density wave and formation of a different correlated state. Using a tight-binding-based approach as well as an effective model, we explain our observations as a consequence of coupling between the single-particle Lifshitz transition during which the Fermi level passes a van Hove singularity and the charge density order. In this scenario, the high electronic density of states associated with the van Hove singularity induces a change in the periodicity of the charge density wave from the known $(3\times 3)$ to a new $(2\times 2)$ superlattice.
format Preprint
id arxiv_https___arxiv_org_abs_2211_01780
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Controlling charge density order in 2H-TaSe$_{2}$ using a van Hove singularity
Luckin, W. R. B.
Li, Y.
Jiang, J.
Gunasekera, S. M.
Wen, C.
Zhang, Y.
Prabhakaran, D.
Flicker, F.
Chen, Y.
Mucha-Kruczynski, M.
Strongly Correlated Electrons
Materials Science
We report on the interplay between a van Hove singularity and a charge density wave state in 2H-TaSe$_{2}$. We use angle-resolved photoemission spectroscopy to investigate changes in the Fermi surface of this material under surface doping with potassium. At high doping, we observe modifications which imply the disappearance of the $(3\times 3)$ charge density wave and formation of a different correlated state. Using a tight-binding-based approach as well as an effective model, we explain our observations as a consequence of coupling between the single-particle Lifshitz transition during which the Fermi level passes a van Hove singularity and the charge density order. In this scenario, the high electronic density of states associated with the van Hove singularity induces a change in the periodicity of the charge density wave from the known $(3\times 3)$ to a new $(2\times 2)$ superlattice.
title Controlling charge density order in 2H-TaSe$_{2}$ using a van Hove singularity
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2211.01780