Tuning metal/superconductor to insulator/superconductor coupling via control of proximity enhancement between NbSe$_2$ monolayers

Fuente: arXiv
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Auteurs principaux: Chiatti, Olivio, Mihov, Klara, Griffin, Theodor U., Grosse, Corinna, Alemayehu, Matti B., Hite, Kyle, Hamann, Danielle, Mogilatenko, Anna, Johnson, David C., Fischer, Saskia F.
Format: Preprint
Publié: 2022
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author Chiatti, Olivio
Mihov, Klara
Griffin, Theodor U.
Grosse, Corinna
Alemayehu, Matti B.
Hite, Kyle
Hamann, Danielle
Mogilatenko, Anna
Johnson, David C.
Fischer, Saskia F.
author_facet Chiatti, Olivio
Mihov, Klara
Griffin, Theodor U.
Grosse, Corinna
Alemayehu, Matti B.
Hite, Kyle
Hamann, Danielle
Mogilatenko, Anna
Johnson, David C.
Fischer, Saskia F.
contents The interplay between charge transfer and electronic disorder in transition-metal dichalcogenide multilayers gives rise to superconductive coupling driven by proximity enhancement, tunneling and superconducting fluctuations, of a yet unwieldy variety. Artificial spacer layers introduced with atomic precision change the density of states by charge transfer. Here, we tune the superconductive coupling between NbSe$_2$ monolayers from proximity-enhanced to tunneling-dominated. We correlate normal and superconducting properties in [(SnSe)$_{1+δ}$]$_m$[NbSe$_2$]$_1$ tailored multilayers with varying SnSe layer thickness. From high-field magnetotransport the critical fields yield Ginzburg-Landau coherence lengths with an increase of 140 % cross-plane , trending towards two-dimensional superconductivity for m > 9. We show cross-over between three regimes: metallic with proximity-enhanced coupling, disordered-metallic with intermediate coupling and insulating with Josephson tunneling. Our results demonstrate that stacking metal mono- and dichalcogenides allows to convert a metal/superconductor into an insulator/superconductor system, prospecting the control of two-dimensional superconductivity in embedded layers.
format Preprint
id arxiv_https___arxiv_org_abs_2212_01084
institution arXiv
publishDate 2022
record_format arxiv
spellingShingle Tuning metal/superconductor to insulator/superconductor coupling via control of proximity enhancement between NbSe$_2$ monolayers
Chiatti, Olivio
Mihov, Klara
Griffin, Theodor U.
Grosse, Corinna
Alemayehu, Matti B.
Hite, Kyle
Hamann, Danielle
Mogilatenko, Anna
Johnson, David C.
Fischer, Saskia F.
Superconductivity
The interplay between charge transfer and electronic disorder in transition-metal dichalcogenide multilayers gives rise to superconductive coupling driven by proximity enhancement, tunneling and superconducting fluctuations, of a yet unwieldy variety. Artificial spacer layers introduced with atomic precision change the density of states by charge transfer. Here, we tune the superconductive coupling between NbSe$_2$ monolayers from proximity-enhanced to tunneling-dominated. We correlate normal and superconducting properties in [(SnSe)$_{1+δ}$]$_m$[NbSe$_2$]$_1$ tailored multilayers with varying SnSe layer thickness. From high-field magnetotransport the critical fields yield Ginzburg-Landau coherence lengths with an increase of 140 % cross-plane , trending towards two-dimensional superconductivity for m > 9. We show cross-over between three regimes: metallic with proximity-enhanced coupling, disordered-metallic with intermediate coupling and insulating with Josephson tunneling. Our results demonstrate that stacking metal mono- and dichalcogenides allows to convert a metal/superconductor into an insulator/superconductor system, prospecting the control of two-dimensional superconductivity in embedded layers.
title Tuning metal/superconductor to insulator/superconductor coupling via control of proximity enhancement between NbSe$_2$ monolayers
topic Superconductivity
url https://arxiv.org/abs/2212.01084