Magneto-optics in a van der Waals magnet tuned by self-hybridized polaritons

Fuente: arXiv
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Autori principali: Dirnberger, Florian, Quan, Jiamin, Bushati, Rezlind, Diederich, Geoffrey, Florian, Matthias, Klein, Julian, Mosina, Kseniia, Sofer, Zdenek, Xu, Xiaodong, Kamra, Akashdeep, García-Vidal, Francisco J., Alù, Andrea, Menon, Vinod M.
Natura: Preprint
Pubblicazione: 2023
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author Dirnberger, Florian
Quan, Jiamin
Bushati, Rezlind
Diederich, Geoffrey
Florian, Matthias
Klein, Julian
Mosina, Kseniia
Sofer, Zdenek
Xu, Xiaodong
Kamra, Akashdeep
García-Vidal, Francisco J.
Alù, Andrea
Menon, Vinod M.
author_facet Dirnberger, Florian
Quan, Jiamin
Bushati, Rezlind
Diederich, Geoffrey
Florian, Matthias
Klein, Julian
Mosina, Kseniia
Sofer, Zdenek
Xu, Xiaodong
Kamra, Akashdeep
García-Vidal, Francisco J.
Alù, Andrea
Menon, Vinod M.
contents Controlling quantum materials with light is of fundamental and technological importance. By utilizing the strong coupling of light and matter in optical cavities (1-3), recent studies were able to modify some of their most defining features (4-6). In this work, we study the magneto-optical properties of a van der Waals magnet that supports strong coupling of photons and excitons even in the absence of external cavity mirrors. In this material - the layered magnetic semiconductor CrSBr - emergent light-matter hybrids called polaritons are shown to significantly increase the spectral bandwidth of correlations between the magnetic, electronic, and optical properties, enabling largely tunable optical responses to applied magnetic fields and magnons. Our results highlight the importance of exciton-photon self-hybridization in van der Waals magnets and motivate novel directions for the manipulation of quantum material properties by strong light-matter coupling.
format Preprint
id arxiv_https___arxiv_org_abs_2301_07593
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Magneto-optics in a van der Waals magnet tuned by self-hybridized polaritons
Dirnberger, Florian
Quan, Jiamin
Bushati, Rezlind
Diederich, Geoffrey
Florian, Matthias
Klein, Julian
Mosina, Kseniia
Sofer, Zdenek
Xu, Xiaodong
Kamra, Akashdeep
García-Vidal, Francisco J.
Alù, Andrea
Menon, Vinod M.
Mesoscale and Nanoscale Physics
Optics
Controlling quantum materials with light is of fundamental and technological importance. By utilizing the strong coupling of light and matter in optical cavities (1-3), recent studies were able to modify some of their most defining features (4-6). In this work, we study the magneto-optical properties of a van der Waals magnet that supports strong coupling of photons and excitons even in the absence of external cavity mirrors. In this material - the layered magnetic semiconductor CrSBr - emergent light-matter hybrids called polaritons are shown to significantly increase the spectral bandwidth of correlations between the magnetic, electronic, and optical properties, enabling largely tunable optical responses to applied magnetic fields and magnons. Our results highlight the importance of exciton-photon self-hybridization in van der Waals magnets and motivate novel directions for the manipulation of quantum material properties by strong light-matter coupling.
title Magneto-optics in a van der Waals magnet tuned by self-hybridized polaritons
topic Mesoscale and Nanoscale Physics
Optics
url https://arxiv.org/abs/2301.07593