Strain-induced dynamic control over the population of quantum emitters in two-dimensional materials
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arXiv
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| Main Authors: | , , , , , , , , , , , , , |
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| Format: | Preprint |
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2023
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| author | Ronco, Giuseppe Martínez-Suárez, Abel Tedeschi, Davide Savaresi, Matteo Hierro-Rodríguez, Aurelio McVitie, Stephen Stroj, Sandra Aberl, Johannes Brehm, Mortiz García-Suárez, Victor M. Rota, Michele B. AlonsoGonzález, Pablo Martín-Sánchez, Javier Trotta, Rinaldo |
| author_facet | Ronco, Giuseppe Martínez-Suárez, Abel Tedeschi, Davide Savaresi, Matteo Hierro-Rodríguez, Aurelio McVitie, Stephen Stroj, Sandra Aberl, Johannes Brehm, Mortiz García-Suárez, Victor M. Rota, Michele B. AlonsoGonzález, Pablo Martín-Sánchez, Javier Trotta, Rinaldo |
| contents | The discovery of quantum emitters (QEs) in two-dimensional materials (2D) has triggered a surge of research to assess their suitability for quantum photonics. While their microscopic origin is still the subject of intense studies, position-controlled QEs are routinely fabricated using static strain gradients, which are used to drive excitons towards localized regions of the crystal where quantum light emission takes place. However, the use of strain in a dynamic fashion to control the brightness of single-photon sources in 2D materials has not been explored so far. In this work, we address this challenge by introducing a novel hybrid semiconductorpiezoelectric device in which WSe2 monolayers are integrated onto piezoelectric pillars that provide both static and dynamic strains. The static strains are first used to induce the formation of QEs, whose emission shows photon anti-bunching. Their energy and brightness are then controlled via the application of voltages to the piezoelectric pillars. Numerical simulations combined with drift-diffusion equations show that these effects are due to a strain-induced modification of the confining-potential landscape, which in turn leads to a net redistribution of excitons among the different QEs. Our work provides a method to dynamically control the brightness of single photon sources based on 2D materials. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2301_10273 |
| institution | arXiv |
| publishDate | 2023 |
| record_format | arxiv |
| spellingShingle | Strain-induced dynamic control over the population of quantum emitters in two-dimensional materials Ronco, Giuseppe Martínez-Suárez, Abel Tedeschi, Davide Savaresi, Matteo Hierro-Rodríguez, Aurelio McVitie, Stephen Stroj, Sandra Aberl, Johannes Brehm, Mortiz García-Suárez, Victor M. Rota, Michele B. AlonsoGonzález, Pablo Martín-Sánchez, Javier Trotta, Rinaldo Materials Science Quantum Physics The discovery of quantum emitters (QEs) in two-dimensional materials (2D) has triggered a surge of research to assess their suitability for quantum photonics. While their microscopic origin is still the subject of intense studies, position-controlled QEs are routinely fabricated using static strain gradients, which are used to drive excitons towards localized regions of the crystal where quantum light emission takes place. However, the use of strain in a dynamic fashion to control the brightness of single-photon sources in 2D materials has not been explored so far. In this work, we address this challenge by introducing a novel hybrid semiconductorpiezoelectric device in which WSe2 monolayers are integrated onto piezoelectric pillars that provide both static and dynamic strains. The static strains are first used to induce the formation of QEs, whose emission shows photon anti-bunching. Their energy and brightness are then controlled via the application of voltages to the piezoelectric pillars. Numerical simulations combined with drift-diffusion equations show that these effects are due to a strain-induced modification of the confining-potential landscape, which in turn leads to a net redistribution of excitons among the different QEs. Our work provides a method to dynamically control the brightness of single photon sources based on 2D materials. |
| title | Strain-induced dynamic control over the population of quantum emitters in two-dimensional materials |
| topic | Materials Science Quantum Physics |
| url | https://arxiv.org/abs/2301.10273 |