Spin waves and orbital contribution to ferromagnetism in a topological metal

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Auteurs principaux: Zhang, Wenliang, Asmara, Teguh Citra, Tseng, Yi, Li, Junbo, Xiong, Yimin, Wei, Yuan, Yu, Tianlun, Galdino, Carlos William, Zhang, Zhijia, Kummer, Kurt, Strocov, Vladimir N., Soh, Y., Schmitt, Thorsten, Aeppli, Gabriel
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Publié: 2023
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author Zhang, Wenliang
Asmara, Teguh Citra
Tseng, Yi
Li, Junbo
Xiong, Yimin
Wei, Yuan
Yu, Tianlun
Galdino, Carlos William
Zhang, Zhijia
Kummer, Kurt
Strocov, Vladimir N.
Soh, Y.
Schmitt, Thorsten
Aeppli, Gabriel
author_facet Zhang, Wenliang
Asmara, Teguh Citra
Tseng, Yi
Li, Junbo
Xiong, Yimin
Wei, Yuan
Yu, Tianlun
Galdino, Carlos William
Zhang, Zhijia
Kummer, Kurt
Strocov, Vladimir N.
Soh, Y.
Schmitt, Thorsten
Aeppli, Gabriel
contents Special arrangements of atoms with more than one atom per unit cell, including honeycomb or kagome (woven bamboo mat) lattices, can host propagating excitations with non-trivial topology as defined by their evolution along closed paths in momentum space. Excitations on such lattices can also be momentum-independent, meaning that they are localized notwithstanding strong hopping of the underlying disturbances between neighbouring sites. The associated flat bands are interesting because the interactions between the heavy quasiparticles inhabiting them will become much more important than for strong dispersion, resulting in novel quantum solid and liquid states. Different stackings of two-dimensional lattices, for example twisted graphene bilayers, provide routes to further engineer topology and many-body effects. Here, we report the discovery, using circularly polarized x-rays for the unambiguous isolation of magnetic signals, of a nearly flat spin wave band and large (compared to elemental iron) orbital moment for the metallic ferromagnet Fe3Sn2, built from compact AB-stacked kagome bilayers and which has a topologically non-trivial electronic band structure controllable by modest external magnetic fields. As a function of out-of-plane momentum, the nearly flat optical mode and the global rotation symmetry-restoring acoustic mode are out of phase, consistent with a bilayer exchange coupling that is larger than the already large in-plane couplings. The defining units of this topological metal are therefore a triangular lattice of octahedral iron clusters rather than weakly coupled kagome planes. The spin waves are strongly damped when compared to elemental iron, opening the topic of interactions of topological bosons (spin waves) and fermions (electrons) with the very specific target of explaining boson lifetimes.
format Preprint
id arxiv_https___arxiv_org_abs_2302_01457
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Spin waves and orbital contribution to ferromagnetism in a topological metal
Zhang, Wenliang
Asmara, Teguh Citra
Tseng, Yi
Li, Junbo
Xiong, Yimin
Wei, Yuan
Yu, Tianlun
Galdino, Carlos William
Zhang, Zhijia
Kummer, Kurt
Strocov, Vladimir N.
Soh, Y.
Schmitt, Thorsten
Aeppli, Gabriel
Strongly Correlated Electrons
Materials Science
Special arrangements of atoms with more than one atom per unit cell, including honeycomb or kagome (woven bamboo mat) lattices, can host propagating excitations with non-trivial topology as defined by their evolution along closed paths in momentum space. Excitations on such lattices can also be momentum-independent, meaning that they are localized notwithstanding strong hopping of the underlying disturbances between neighbouring sites. The associated flat bands are interesting because the interactions between the heavy quasiparticles inhabiting them will become much more important than for strong dispersion, resulting in novel quantum solid and liquid states. Different stackings of two-dimensional lattices, for example twisted graphene bilayers, provide routes to further engineer topology and many-body effects. Here, we report the discovery, using circularly polarized x-rays for the unambiguous isolation of magnetic signals, of a nearly flat spin wave band and large (compared to elemental iron) orbital moment for the metallic ferromagnet Fe3Sn2, built from compact AB-stacked kagome bilayers and which has a topologically non-trivial electronic band structure controllable by modest external magnetic fields. As a function of out-of-plane momentum, the nearly flat optical mode and the global rotation symmetry-restoring acoustic mode are out of phase, consistent with a bilayer exchange coupling that is larger than the already large in-plane couplings. The defining units of this topological metal are therefore a triangular lattice of octahedral iron clusters rather than weakly coupled kagome planes. The spin waves are strongly damped when compared to elemental iron, opening the topic of interactions of topological bosons (spin waves) and fermions (electrons) with the very specific target of explaining boson lifetimes.
title Spin waves and orbital contribution to ferromagnetism in a topological metal
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2302.01457