Instability of the charge density wave in Kagome magnet FeGe

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Hauptverfasser: Chen, Ziyuan, Wu, Xueliang, Yin, Ruotong, Zhang, Jiakang, Wang, Shiyuan, Li, Yuanji, Li, Mingzhe, Wang, Aifeng, Wang, Yilin, Yan, Ya-Jun, Feng, Dong-Lai
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Veröffentlicht: 2023
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author Chen, Ziyuan
Wu, Xueliang
Yin, Ruotong
Zhang, Jiakang
Wang, Shiyuan
Li, Yuanji
Li, Mingzhe
Wang, Aifeng
Wang, Yilin
Yan, Ya-Jun
Feng, Dong-Lai
author_facet Chen, Ziyuan
Wu, Xueliang
Yin, Ruotong
Zhang, Jiakang
Wang, Shiyuan
Li, Yuanji
Li, Mingzhe
Wang, Aifeng
Wang, Yilin
Yan, Ya-Jun
Feng, Dong-Lai
contents Kagome metals show rich competing quantum phases due to geometry frustration, flat bands, many-body effects, and non-trivial topology. Recently, a novel charge density wave (CDW) was discovered deep inside the antiferromagnetic phase of FeGe, attracting intense attention due to close relation with magnetism. Here, via a scanning tunneling microscope (STM), we find the 2*2 CDW in FeGe is very fragile and can be readily disrupted into the initial 1*1 phase; Small sqrt3*sqrt3 CDW puddles are found to coexist with the 2*2 CDW in as-grown samples, and can also be induced in the intermediate process of CDW disruption, which will eventually transform into the initial 1*1 phase. Moreover, an exotic intermediate CDW state and standalone CDW nuclei appear unexpectedly during the disruption process. Our first-principle calculations find equal softening of a flat optical phonon mode in a large momentum region around the CDW wave vector, corresponding to numerous competing CDWs with close energies. This might lead to strong instability of the CDW ground state, responsible for STM observations. Our findings provide more novel experimental aspects to understand the CDW in FeGe and suggest FeGe-like Kagome metals are ideal platforms for studying the physics of competing CDW instabilities.
format Preprint
id arxiv_https___arxiv_org_abs_2302_04490
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Instability of the charge density wave in Kagome magnet FeGe
Chen, Ziyuan
Wu, Xueliang
Yin, Ruotong
Zhang, Jiakang
Wang, Shiyuan
Li, Yuanji
Li, Mingzhe
Wang, Aifeng
Wang, Yilin
Yan, Ya-Jun
Feng, Dong-Lai
Strongly Correlated Electrons
Materials Science
Kagome metals show rich competing quantum phases due to geometry frustration, flat bands, many-body effects, and non-trivial topology. Recently, a novel charge density wave (CDW) was discovered deep inside the antiferromagnetic phase of FeGe, attracting intense attention due to close relation with magnetism. Here, via a scanning tunneling microscope (STM), we find the 2*2 CDW in FeGe is very fragile and can be readily disrupted into the initial 1*1 phase; Small sqrt3*sqrt3 CDW puddles are found to coexist with the 2*2 CDW in as-grown samples, and can also be induced in the intermediate process of CDW disruption, which will eventually transform into the initial 1*1 phase. Moreover, an exotic intermediate CDW state and standalone CDW nuclei appear unexpectedly during the disruption process. Our first-principle calculations find equal softening of a flat optical phonon mode in a large momentum region around the CDW wave vector, corresponding to numerous competing CDWs with close energies. This might lead to strong instability of the CDW ground state, responsible for STM observations. Our findings provide more novel experimental aspects to understand the CDW in FeGe and suggest FeGe-like Kagome metals are ideal platforms for studying the physics of competing CDW instabilities.
title Instability of the charge density wave in Kagome magnet FeGe
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2302.04490