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Bibliographic Details
Main Authors: Cheng, Guanjian, Gong, Xin-Gao, Yin, Wan-Jian
Format: Preprint
Published: 2023
Subjects:
Online Access:https://arxiv.org/abs/2302.13537
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Table of Contents:
  • We introduce a computational method to optimize target physical properties in the full configuration space regarding atomic composition, chemical stoichiometry, and crystal structure. The approach combines the universal potential of the crystal graph neural network and Bayesian optimization. The proposed approach effectively obtains the crystal structure with the strongest atomic cohesion from all possible crystals. Several new crystals with high atomic cohesion are identified and confirmed by density functional theory for thermodynamic and dynamic stability. Our method introduces a novel approach to inverse materials design with additional functional properties for practical applications.