Axion optical induction of antiferromagnetic order

Fuente: arXiv
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Autori principali: Qiu, Jian-Xiang, Tzschaschel, Christian, Ahn, Junyeong, Gao, Anyuan, Li, Houchen, Zhang, Xin-Yue, Ghosh, Barun, Hu, Chaowei, Wang, Yu-Xuan, Liu, Yu-Fei, Bérubé, Damien, Dinh, Thao, Gong, Zhenhao, Lien, Shang-Wei, Ho, Sheng-Chin, Singh, Bahadur, Watanabe, Kenji, Taniguchi, Takashi, Bell, David C., Lu, Hai-Zhou, Bansil, Arun, Lin, Hsin, Chang, Tay-Rong, Zhou, Brian B., Ma, Qiong, Vishwanath, Ashvin, Ni, Ni, Xu, Su-Yang
Natura: Preprint
Pubblicazione: 2023
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author Qiu, Jian-Xiang
Tzschaschel, Christian
Ahn, Junyeong
Gao, Anyuan
Li, Houchen
Zhang, Xin-Yue
Ghosh, Barun
Hu, Chaowei
Wang, Yu-Xuan
Liu, Yu-Fei
Bérubé, Damien
Dinh, Thao
Gong, Zhenhao
Lien, Shang-Wei
Ho, Sheng-Chin
Singh, Bahadur
Watanabe, Kenji
Taniguchi, Takashi
Bell, David C.
Lu, Hai-Zhou
Bansil, Arun
Lin, Hsin
Chang, Tay-Rong
Zhou, Brian B.
Ma, Qiong
Vishwanath, Ashvin
Ni, Ni
Xu, Su-Yang
author_facet Qiu, Jian-Xiang
Tzschaschel, Christian
Ahn, Junyeong
Gao, Anyuan
Li, Houchen
Zhang, Xin-Yue
Ghosh, Barun
Hu, Chaowei
Wang, Yu-Xuan
Liu, Yu-Fei
Bérubé, Damien
Dinh, Thao
Gong, Zhenhao
Lien, Shang-Wei
Ho, Sheng-Chin
Singh, Bahadur
Watanabe, Kenji
Taniguchi, Takashi
Bell, David C.
Lu, Hai-Zhou
Bansil, Arun
Lin, Hsin
Chang, Tay-Rong
Zhou, Brian B.
Ma, Qiong
Vishwanath, Ashvin
Ni, Ni
Xu, Su-Yang
contents Using circularly-polarized light to control quantum matter is a highly intriguing topic in physics, chemistry and biology. Previous studies have demonstrated helicity-dependent optical control of spatial chirality and magnetization $M$. The former is central for asymmetric synthesis in chemistry and homochirality in bio-molecules, while the latter is of great interest for ferromagnetic spintronics. In this paper, we report the surprising observation of helicity-dependent optical control of fully-compensated antiferromagnetic (AFM) order in 2D even-layered MnBi$_2$Te$_4$, a topological Axion insulator with neither chirality nor $M$. We further demonstrate helicity-dependent optical creation of AFM domain walls by double induction beams and the direct reversal of AFM domains by ultrafast pulses. The control and reversal of AFM domains and domain walls by light helicity have never been achieved in any fully-compensated AFM. To understand this optical control, we study a novel type of circular dichroism (CD) proportional to the AFM order, which only appears in reflection but is absent in transmission. We show that the optical control and CD both arise from the optical Axion electrodynamics, which can be visualized as a Berry curvature real space dipole. Our Axion induction provides the possibility to optically control a family of $\mathcal{PT}$-symmetric AFMs such as Cr$_2$O$_3$, CrI$_3$ and possibly novel states in cuprates. In MnBi$_2$Te$_4$, this further opens the door for optical writing of dissipationless circuit formed by topological edge states.
format Preprint
id arxiv_https___arxiv_org_abs_2303_05451
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Axion optical induction of antiferromagnetic order
Qiu, Jian-Xiang
Tzschaschel, Christian
Ahn, Junyeong
Gao, Anyuan
Li, Houchen
Zhang, Xin-Yue
Ghosh, Barun
Hu, Chaowei
Wang, Yu-Xuan
Liu, Yu-Fei
Bérubé, Damien
Dinh, Thao
Gong, Zhenhao
Lien, Shang-Wei
Ho, Sheng-Chin
Singh, Bahadur
Watanabe, Kenji
Taniguchi, Takashi
Bell, David C.
Lu, Hai-Zhou
Bansil, Arun
Lin, Hsin
Chang, Tay-Rong
Zhou, Brian B.
Ma, Qiong
Vishwanath, Ashvin
Ni, Ni
Xu, Su-Yang
Mesoscale and Nanoscale Physics
Materials Science
High Energy Physics - Phenomenology
Using circularly-polarized light to control quantum matter is a highly intriguing topic in physics, chemistry and biology. Previous studies have demonstrated helicity-dependent optical control of spatial chirality and magnetization $M$. The former is central for asymmetric synthesis in chemistry and homochirality in bio-molecules, while the latter is of great interest for ferromagnetic spintronics. In this paper, we report the surprising observation of helicity-dependent optical control of fully-compensated antiferromagnetic (AFM) order in 2D even-layered MnBi$_2$Te$_4$, a topological Axion insulator with neither chirality nor $M$. We further demonstrate helicity-dependent optical creation of AFM domain walls by double induction beams and the direct reversal of AFM domains by ultrafast pulses. The control and reversal of AFM domains and domain walls by light helicity have never been achieved in any fully-compensated AFM. To understand this optical control, we study a novel type of circular dichroism (CD) proportional to the AFM order, which only appears in reflection but is absent in transmission. We show that the optical control and CD both arise from the optical Axion electrodynamics, which can be visualized as a Berry curvature real space dipole. Our Axion induction provides the possibility to optically control a family of $\mathcal{PT}$-symmetric AFMs such as Cr$_2$O$_3$, CrI$_3$ and possibly novel states in cuprates. In MnBi$_2$Te$_4$, this further opens the door for optical writing of dissipationless circuit formed by topological edge states.
title Axion optical induction of antiferromagnetic order
topic Mesoscale and Nanoscale Physics
Materials Science
High Energy Physics - Phenomenology
url https://arxiv.org/abs/2303.05451