Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene

Fuente: arXiv
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Main Authors: Kwan, Yves H., Wagner, Glenn, Bultinck, Nick, Simon, Steven H., Berg, Erez, Parameswaran, S. A.
Format: Preprint
Published: 2023
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author Kwan, Yves H.
Wagner, Glenn
Bultinck, Nick
Simon, Steven H.
Berg, Erez
Parameswaran, S. A.
author_facet Kwan, Yves H.
Wagner, Glenn
Bultinck, Nick
Simon, Steven H.
Berg, Erez
Parameswaran, S. A.
contents Recent scanning tunneling microscopy experiments [K.P. Nuckolls et al., arXiv:2303.00024] have revealed the ubiquity of Kekulé charge-density wave order in magic-angle twisted bilayer graphene. Most samples are moderately strained and show `incommensurate Kekulé spiral' (IKS) order involving a graphene-scale charge density distortion uniaxially modulated on the scale of the moiré superlattice, in accord with theoretical predictions. However, ultra-low strain samples instead show graphene-scale Kekulé charge order that is uniform on the moiré scale. This order, especially prominent near filling factor $ν=-2$, is unanticipated by theory which predicts a time-reversal breaking Kekulé current order at low strain. We show that including the coupling of moiré electrons to graphene-scale optical zone-corner (ZC) phonons stabilizes a uniform Kekulé charge ordered state at $|ν|=2$ with a quantized topological (spin or anomalous Hall) response. Our work clarifies how this phonon-driven selection of electronic order emerges in the strong-coupling regime of moiré graphene.
format Preprint
id arxiv_https___arxiv_org_abs_2303_13602
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene
Kwan, Yves H.
Wagner, Glenn
Bultinck, Nick
Simon, Steven H.
Berg, Erez
Parameswaran, S. A.
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Recent scanning tunneling microscopy experiments [K.P. Nuckolls et al., arXiv:2303.00024] have revealed the ubiquity of Kekulé charge-density wave order in magic-angle twisted bilayer graphene. Most samples are moderately strained and show `incommensurate Kekulé spiral' (IKS) order involving a graphene-scale charge density distortion uniaxially modulated on the scale of the moiré superlattice, in accord with theoretical predictions. However, ultra-low strain samples instead show graphene-scale Kekulé charge order that is uniform on the moiré scale. This order, especially prominent near filling factor $ν=-2$, is unanticipated by theory which predicts a time-reversal breaking Kekulé current order at low strain. We show that including the coupling of moiré electrons to graphene-scale optical zone-corner (ZC) phonons stabilizes a uniform Kekulé charge ordered state at $|ν|=2$ with a quantized topological (spin or anomalous Hall) response. Our work clarifies how this phonon-driven selection of electronic order emerges in the strong-coupling regime of moiré graphene.
title Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2303.13602