Measurement principles for quantum spectroscopy of molecular materials with entangled photons
Fuente:
arXiv
Saved in:
| Main Authors: | , , , , , , , , , , |
|---|---|
| Format: | Preprint |
| Published: |
2023
|
| Subjects: | |
| Online Access: | |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| _version_ | 1866909111639080960 |
|---|---|
| author | Moretti, Luca Rojas-Gatjens, Esteban Uboldi, Lorenzo Tiede, David Otto Kumar, Evan J Trovatello, Chiara Preda, Fabrizio Perri, Antonio Manzoni, Cristian Cerullo, Giulio Kandada, Ajay Ram Srimath |
| author_facet | Moretti, Luca Rojas-Gatjens, Esteban Uboldi, Lorenzo Tiede, David Otto Kumar, Evan J Trovatello, Chiara Preda, Fabrizio Perri, Antonio Manzoni, Cristian Cerullo, Giulio Kandada, Ajay Ram Srimath |
| contents | Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose however lack the frequency tunability and spectral bandwidth demanded by contemporary molecular materials. Here, we present design strategies for efficient spontaneous parametric downconversion to generate biphoton states with adequate spectral bandwidth and at visible wavelengths. Importantly, we demonstrate, by suitable design of the nonlinear optical interaction, the scope to engineer the degree of spectral correlations between the photons of the pair. We also present an experimental methodology to effectively characterize such spectral correlations. Importantly, we believe that such a characterization tool can be effectively adapted as a spectroscopy platform to optically probe system-bath interactions in materials. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2304_07828 |
| institution | arXiv |
| publishDate | 2023 |
| record_format | arxiv |
| spellingShingle | Measurement principles for quantum spectroscopy of molecular materials with entangled photons Moretti, Luca Rojas-Gatjens, Esteban Uboldi, Lorenzo Tiede, David Otto Kumar, Evan J Trovatello, Chiara Preda, Fabrizio Perri, Antonio Manzoni, Cristian Cerullo, Giulio Kandada, Ajay Ram Srimath Optics Chemical Physics Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose however lack the frequency tunability and spectral bandwidth demanded by contemporary molecular materials. Here, we present design strategies for efficient spontaneous parametric downconversion to generate biphoton states with adequate spectral bandwidth and at visible wavelengths. Importantly, we demonstrate, by suitable design of the nonlinear optical interaction, the scope to engineer the degree of spectral correlations between the photons of the pair. We also present an experimental methodology to effectively characterize such spectral correlations. Importantly, we believe that such a characterization tool can be effectively adapted as a spectroscopy platform to optically probe system-bath interactions in materials. |
| title | Measurement principles for quantum spectroscopy of molecular materials with entangled photons |
| topic | Optics Chemical Physics |
| url | https://arxiv.org/abs/2304.07828 |