Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moiré $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer

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Main Authors: Gao, Beini, Suárez-Forero, Daniel G., Sarkar, Supratik, Huang, Tsung-Sheng, Session, Deric, Mehrabad, Mahmoud Jalali, Ni, Ruihao, Xie, Ming, Upadhyay, Pranshoo, Vannucci, Jonathan, Mittal, Sunil, Watanabe, Kenji, Taniguchi, Takashi, Imamoglu, Atac, Zhou, You, Hafezi, Mohammad
Format: Preprint
Published: 2023
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author Gao, Beini
Suárez-Forero, Daniel G.
Sarkar, Supratik
Huang, Tsung-Sheng
Session, Deric
Mehrabad, Mahmoud Jalali
Ni, Ruihao
Xie, Ming
Upadhyay, Pranshoo
Vannucci, Jonathan
Mittal, Sunil
Watanabe, Kenji
Taniguchi, Takashi
Imamoglu, Atac
Zhou, You
Hafezi, Mohammad
author_facet Gao, Beini
Suárez-Forero, Daniel G.
Sarkar, Supratik
Huang, Tsung-Sheng
Session, Deric
Mehrabad, Mahmoud Jalali
Ni, Ruihao
Xie, Ming
Upadhyay, Pranshoo
Vannucci, Jonathan
Mittal, Sunil
Watanabe, Kenji
Taniguchi, Takashi
Imamoglu, Atac
Zhou, You
Hafezi, Mohammad
contents Understanding the Hubbard model is crucial for investigating various quantum many-body states and its fermionic and bosonic versions have been largely realized separately. Recently, transition metal dichalcogenides heterobilayers have emerged as a promising platform for simulating the rich physics of the Hubbard model. In this work, we explore the interplay between fermionic and bosonic populations, using a $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer device that hosts this hybrid particle density. We independently tune the fermionic and bosonic populations by electronic doping and optical injection of electron-hole pairs, respectively. This enables us to form strongly interacting excitons that are manifested in a large energy gap in the photoluminescence spectrum. The incompressibility of excitons is further corroborated by measuring exciton diffusion, which remains constant upon increasing pumping intensity, as opposed to the expected behavior of a weakly interacting gas of bosons, suggesting the formation of a bosonic Mott insulator. We explain our observations using a two-band model including phase space filling. Our system provides a controllable approach to the exploration of quantum many-body effects in the generalized Bose-Fermi-Hubbard model.
format Preprint
id arxiv_https___arxiv_org_abs_2304_09731
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moiré $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer
Gao, Beini
Suárez-Forero, Daniel G.
Sarkar, Supratik
Huang, Tsung-Sheng
Session, Deric
Mehrabad, Mahmoud Jalali
Ni, Ruihao
Xie, Ming
Upadhyay, Pranshoo
Vannucci, Jonathan
Mittal, Sunil
Watanabe, Kenji
Taniguchi, Takashi
Imamoglu, Atac
Zhou, You
Hafezi, Mohammad
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Quantum Physics
Understanding the Hubbard model is crucial for investigating various quantum many-body states and its fermionic and bosonic versions have been largely realized separately. Recently, transition metal dichalcogenides heterobilayers have emerged as a promising platform for simulating the rich physics of the Hubbard model. In this work, we explore the interplay between fermionic and bosonic populations, using a $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer device that hosts this hybrid particle density. We independently tune the fermionic and bosonic populations by electronic doping and optical injection of electron-hole pairs, respectively. This enables us to form strongly interacting excitons that are manifested in a large energy gap in the photoluminescence spectrum. The incompressibility of excitons is further corroborated by measuring exciton diffusion, which remains constant upon increasing pumping intensity, as opposed to the expected behavior of a weakly interacting gas of bosons, suggesting the formation of a bosonic Mott insulator. We explain our observations using a two-band model including phase space filling. Our system provides a controllable approach to the exploration of quantum many-body effects in the generalized Bose-Fermi-Hubbard model.
title Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moiré $\rm{WS}_2$/$\rm{WSe}_2$ heterobilayer
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Quantum Physics
url https://arxiv.org/abs/2304.09731