Photostrictive actuators based on freestanding ferroelectric membranes

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Ganguly, Saptam, Pesquera, David, Garcia, Daniel Moreno, Saeed, Umair, Mirzamohammadi, Nona, Santiso, José, Padilla, Jessica, Roque, José Manuel Caicedo, Laulhé, Claire, Berenguer, Felisa, Villanueva, Luis Guillermo, Catalan, Gustau
Format: Preprint
Published: 2023
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866909749882126336
author Ganguly, Saptam
Pesquera, David
Garcia, Daniel Moreno
Saeed, Umair
Mirzamohammadi, Nona
Santiso, José
Padilla, Jessica
Roque, José Manuel Caicedo
Laulhé, Claire
Berenguer, Felisa
Villanueva, Luis Guillermo
Catalan, Gustau
author_facet Ganguly, Saptam
Pesquera, David
Garcia, Daniel Moreno
Saeed, Umair
Mirzamohammadi, Nona
Santiso, José
Padilla, Jessica
Roque, José Manuel Caicedo
Laulhé, Claire
Berenguer, Felisa
Villanueva, Luis Guillermo
Catalan, Gustau
contents Complex oxides offer a wide range of functional properties, and recent advances in fabrication of freestanding membranes of these oxides are adding new mechanical degrees of freedom to this already rich functional ecosystem. Here, we demonstrate photoactuation in freestanding thin film resonators of ferroelectric Barium Titanate (BaTiO3) and paraelectric Strontium Titanate (SrTiO3). The free-standing films, transferred onto perforated supports, act as nano-drums, oscillating at their natural resonance frequency when illuminated by a frequency-modulated laser. The light-induced deflections in the ferroelectric BaTiO3 membranes are two orders of magnitude larger than in the paraelectric SrTiO3 ones. Time-resolved X-ray micro-diffraction under illumination and temperature-dependent and holographic interferometry provide combined evidence for the photostrictive strain in BaTiO3 originating from partial screening of ferroelectric polarization by photo-excited carriers, which decreases the tetragonality of the unit cell. These findings showcase the potential of photostrictive freestanding ferroelectric films as wireless actuators operated by light.
format Preprint
id arxiv_https___arxiv_org_abs_2305_03193
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Photostrictive actuators based on freestanding ferroelectric membranes
Ganguly, Saptam
Pesquera, David
Garcia, Daniel Moreno
Saeed, Umair
Mirzamohammadi, Nona
Santiso, José
Padilla, Jessica
Roque, José Manuel Caicedo
Laulhé, Claire
Berenguer, Felisa
Villanueva, Luis Guillermo
Catalan, Gustau
Materials Science
Applied Physics
Complex oxides offer a wide range of functional properties, and recent advances in fabrication of freestanding membranes of these oxides are adding new mechanical degrees of freedom to this already rich functional ecosystem. Here, we demonstrate photoactuation in freestanding thin film resonators of ferroelectric Barium Titanate (BaTiO3) and paraelectric Strontium Titanate (SrTiO3). The free-standing films, transferred onto perforated supports, act as nano-drums, oscillating at their natural resonance frequency when illuminated by a frequency-modulated laser. The light-induced deflections in the ferroelectric BaTiO3 membranes are two orders of magnitude larger than in the paraelectric SrTiO3 ones. Time-resolved X-ray micro-diffraction under illumination and temperature-dependent and holographic interferometry provide combined evidence for the photostrictive strain in BaTiO3 originating from partial screening of ferroelectric polarization by photo-excited carriers, which decreases the tetragonality of the unit cell. These findings showcase the potential of photostrictive freestanding ferroelectric films as wireless actuators operated by light.
title Photostrictive actuators based on freestanding ferroelectric membranes
topic Materials Science
Applied Physics
url https://arxiv.org/abs/2305.03193