Chiral excitations and the intermediate-field spin-liquid regime in the Kitaev magnet $α$-RuCl$_3$

Fuente: arXiv
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Auteurs principaux: Sahasrabudhe, Anuja, Prosnikov, Mikhail A., Koethe, Thomas C., Stein, Philipp, Tsurkan, Vladimir, Loidl, Alois, Grüninger, Markus, Hedayat, Hamoon, van Loosdrecht, Paul H. M.
Format: Preprint
Publié: 2023
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author Sahasrabudhe, Anuja
Prosnikov, Mikhail A.
Koethe, Thomas C.
Stein, Philipp
Tsurkan, Vladimir
Loidl, Alois
Grüninger, Markus
Hedayat, Hamoon
van Loosdrecht, Paul H. M.
author_facet Sahasrabudhe, Anuja
Prosnikov, Mikhail A.
Koethe, Thomas C.
Stein, Philipp
Tsurkan, Vladimir
Loidl, Alois
Grüninger, Markus
Hedayat, Hamoon
van Loosdrecht, Paul H. M.
contents In the Kitaev magnet $α$-RuCl$_3$, the existence of a magnetic-field-induced quantum spin liquid phase and of anyonic excitations are discussed controversially. We address this elusive, exotic phase via helicity-dependent Raman scattering and analyze the Raman optical activity of excitations as a function of magnetic field and temperature. The hotly debated field regime between 7.5 T and 10.5 T is characterized by clear spectroscopic signatures such as a plateau of the Raman optical activity of the dominant, chiral spin-flip excitation. This provides direct evidence for the existence of a distinct intermediate field regime compatible with a quantum spin liquid phase.
format Preprint
id arxiv_https___arxiv_org_abs_2305_03400
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Chiral excitations and the intermediate-field spin-liquid regime in the Kitaev magnet $α$-RuCl$_3$
Sahasrabudhe, Anuja
Prosnikov, Mikhail A.
Koethe, Thomas C.
Stein, Philipp
Tsurkan, Vladimir
Loidl, Alois
Grüninger, Markus
Hedayat, Hamoon
van Loosdrecht, Paul H. M.
Strongly Correlated Electrons
In the Kitaev magnet $α$-RuCl$_3$, the existence of a magnetic-field-induced quantum spin liquid phase and of anyonic excitations are discussed controversially. We address this elusive, exotic phase via helicity-dependent Raman scattering and analyze the Raman optical activity of excitations as a function of magnetic field and temperature. The hotly debated field regime between 7.5 T and 10.5 T is characterized by clear spectroscopic signatures such as a plateau of the Raman optical activity of the dominant, chiral spin-flip excitation. This provides direct evidence for the existence of a distinct intermediate field regime compatible with a quantum spin liquid phase.
title Chiral excitations and the intermediate-field spin-liquid regime in the Kitaev magnet $α$-RuCl$_3$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2305.03400