Optically addressable spin defects coupled to bound states in the continuum metasurfaces

Fuente: arXiv
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Main Authors: Sortino, Luca, Gale, Angus, Kühner, Lucca, Li, Chi, Biechteler, Jonas, Wendisch, Fedja J., Kianinia, Mehran, Ren, Haoran, Toth, Milos, Maier, Stefan A., Aharonovich, Igor, Tittl, Andreas
Format: Preprint
Published: 2023
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author Sortino, Luca
Gale, Angus
Kühner, Lucca
Li, Chi
Biechteler, Jonas
Wendisch, Fedja J.
Kianinia, Mehran
Ren, Haoran
Toth, Milos
Maier, Stefan A.
Aharonovich, Igor
Tittl, Andreas
author_facet Sortino, Luca
Gale, Angus
Kühner, Lucca
Li, Chi
Biechteler, Jonas
Wendisch, Fedja J.
Kianinia, Mehran
Ren, Haoran
Toth, Milos
Maier, Stefan A.
Aharonovich, Igor
Tittl, Andreas
contents Van der Waals (vdW) materials, including hexagonal boron nitride (hBN), are layered crystalline solids with appealing properties for investigating light-matter interactions at the nanoscale. hBN has emerged as a versatile building block for nanophotonic structures, and the recent identification of native optically addressable spin defects has opened up exciting possibilities in quantum technologies. However, these defects exhibit relatively low quantum efficiencies and a broad emission spectrum, limiting potential applications. Optical metasurfaces present a novel approach to boost light emission efficiency, offering remarkable control over light-matter coupling at the sub-wavelength regime. Here, we propose and realise a monolithic scalable integration between intrinsic spin defects in hBN metasurfaces and high quality (Q) factor resonances leveraging quasi-bound states in the continuum (qBICs). Coupling between spin defect ensembles and qBIC resonances delivers a 25-fold increase in photoluminescence intensity, accompanied by spectral narrowing to below 4 nm linewidth facilitated by Q factors exceeding $10^2$. Our findings demonstrate a new class of spin based metasurfaces and pave the way towards vdW-based nanophotonic devices with enhanced efficiency and sensitivity for quantum applications in imaging, sensing, and light emission.
format Preprint
id arxiv_https___arxiv_org_abs_2306_05735
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Optically addressable spin defects coupled to bound states in the continuum metasurfaces
Sortino, Luca
Gale, Angus
Kühner, Lucca
Li, Chi
Biechteler, Jonas
Wendisch, Fedja J.
Kianinia, Mehran
Ren, Haoran
Toth, Milos
Maier, Stefan A.
Aharonovich, Igor
Tittl, Andreas
Optics
Mesoscale and Nanoscale Physics
Van der Waals (vdW) materials, including hexagonal boron nitride (hBN), are layered crystalline solids with appealing properties for investigating light-matter interactions at the nanoscale. hBN has emerged as a versatile building block for nanophotonic structures, and the recent identification of native optically addressable spin defects has opened up exciting possibilities in quantum technologies. However, these defects exhibit relatively low quantum efficiencies and a broad emission spectrum, limiting potential applications. Optical metasurfaces present a novel approach to boost light emission efficiency, offering remarkable control over light-matter coupling at the sub-wavelength regime. Here, we propose and realise a monolithic scalable integration between intrinsic spin defects in hBN metasurfaces and high quality (Q) factor resonances leveraging quasi-bound states in the continuum (qBICs). Coupling between spin defect ensembles and qBIC resonances delivers a 25-fold increase in photoluminescence intensity, accompanied by spectral narrowing to below 4 nm linewidth facilitated by Q factors exceeding $10^2$. Our findings demonstrate a new class of spin based metasurfaces and pave the way towards vdW-based nanophotonic devices with enhanced efficiency and sensitivity for quantum applications in imaging, sensing, and light emission.
title Optically addressable spin defects coupled to bound states in the continuum metasurfaces
topic Optics
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2306.05735