Magnetic structure and Kondo lattice behavior in CeVGe$_3$: an NMR and neutron scattering study

Fuente: arXiv
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Main Authors: Chaffey, C., Wu, H. C., Jin, Hanshang, Sherpa, P., Klavins, Peter, Avdeev, M., Aji, S., Shimodate, R., Nawa, K., Sato, T. J., Taufour, V., Curro, N. J.
Format: Preprint
Published: 2023
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author Chaffey, C.
Wu, H. C.
Jin, Hanshang
Sherpa, P.
Klavins, Peter
Avdeev, M.
Aji, S.
Shimodate, R.
Nawa, K.
Sato, T. J.
Taufour, V.
Curro, N. J.
author_facet Chaffey, C.
Wu, H. C.
Jin, Hanshang
Sherpa, P.
Klavins, Peter
Avdeev, M.
Aji, S.
Shimodate, R.
Nawa, K.
Sato, T. J.
Taufour, V.
Curro, N. J.
contents We present nuclear magnetic resonance (NMR), neutron diffraction, magnetization, and transport measurements on a single crystal and powder of CeVGe$_3$. This material exhibits heavy fermion behavior at low temperature, accompanied by antiferromagnetic (AFM) order below 5.8 K. We find that the magnetic structure is incommensurate with AFM helical structure, characterized by a magnetic modulated propagation vector of $(0, 0, 0.49)$ with in-plane moments rotating around the $c$-axis. The NMR Knight shift and spin-lattice relaxation rate reveal a coherence temperature $T^*\sim 15$ K, and the presence of significant antiferromagnetic fluctuations reminiscent of the archetypical heavy fermion compound CeRhIn$_5$. We further identify a metamagnetic transition above $H_m\sim 2.5$ T for magnetic fields perpendicular to $c$. We speculate that the magnetic structure in this field-induced phase consists of a superposition with both ferromagnetic and antiferromagnetic components, which is consistent with the NMR spectrum in this region of the phase diagram. Our results thus indicate that CeVGe$_3$ is a hexagonal structure analog to tetragonal CeRhIn$_5$.
format Preprint
id arxiv_https___arxiv_org_abs_2306_10166
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Magnetic structure and Kondo lattice behavior in CeVGe$_3$: an NMR and neutron scattering study
Chaffey, C.
Wu, H. C.
Jin, Hanshang
Sherpa, P.
Klavins, Peter
Avdeev, M.
Aji, S.
Shimodate, R.
Nawa, K.
Sato, T. J.
Taufour, V.
Curro, N. J.
Strongly Correlated Electrons
We present nuclear magnetic resonance (NMR), neutron diffraction, magnetization, and transport measurements on a single crystal and powder of CeVGe$_3$. This material exhibits heavy fermion behavior at low temperature, accompanied by antiferromagnetic (AFM) order below 5.8 K. We find that the magnetic structure is incommensurate with AFM helical structure, characterized by a magnetic modulated propagation vector of $(0, 0, 0.49)$ with in-plane moments rotating around the $c$-axis. The NMR Knight shift and spin-lattice relaxation rate reveal a coherence temperature $T^*\sim 15$ K, and the presence of significant antiferromagnetic fluctuations reminiscent of the archetypical heavy fermion compound CeRhIn$_5$. We further identify a metamagnetic transition above $H_m\sim 2.5$ T for magnetic fields perpendicular to $c$. We speculate that the magnetic structure in this field-induced phase consists of a superposition with both ferromagnetic and antiferromagnetic components, which is consistent with the NMR spectrum in this region of the phase diagram. Our results thus indicate that CeVGe$_3$ is a hexagonal structure analog to tetragonal CeRhIn$_5$.
title Magnetic structure and Kondo lattice behavior in CeVGe$_3$: an NMR and neutron scattering study
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2306.10166