Zinc blende ZnS (001) surface structure investigated by XPS,LEED and DFT

Fuente: arXiv
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Auteurs principaux: Oliveira, Pablo, Arrouvel, Corinne, Stavale, Fernando
Format: Preprint
Publié: 2023
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_version_ 1866929724305965056
author Oliveira, Pablo
Arrouvel, Corinne
Stavale, Fernando
author_facet Oliveira, Pablo
Arrouvel, Corinne
Stavale, Fernando
contents The formation and stability of a sulfur-rich surface of the zinc blende ZnS (001) single crystal have been examined by x-ray photoemission spectroscopy (XPS), low-energy electron diffraction (LEED), and density-functional theory (DFT) calculations. LEED patterns obtained from ZnS (001) surface prepared in ultrahigh vacuum conditions are compatible to the formation of the ($1 \times 2$) reconstruction. Further XPS investigation is consistent with the conversion of the surface region into a sulfur-rich surface. DFT calculations support the S-richer ZnS surface hypothesis and the indirect notion of increasing in the conductivity of such a new structure.
format Preprint
id arxiv_https___arxiv_org_abs_2307_06549
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Zinc blende ZnS (001) surface structure investigated by XPS,LEED and DFT
Oliveira, Pablo
Arrouvel, Corinne
Stavale, Fernando
Materials Science
The formation and stability of a sulfur-rich surface of the zinc blende ZnS (001) single crystal have been examined by x-ray photoemission spectroscopy (XPS), low-energy electron diffraction (LEED), and density-functional theory (DFT) calculations. LEED patterns obtained from ZnS (001) surface prepared in ultrahigh vacuum conditions are compatible to the formation of the ($1 \times 2$) reconstruction. Further XPS investigation is consistent with the conversion of the surface region into a sulfur-rich surface. DFT calculations support the S-richer ZnS surface hypothesis and the indirect notion of increasing in the conductivity of such a new structure.
title Zinc blende ZnS (001) surface structure investigated by XPS,LEED and DFT
topic Materials Science
url https://arxiv.org/abs/2307.06549