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| Main Authors: | , , , , , , , , , , , , , |
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| Format: | Preprint |
| Published: |
2023
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| Subjects: | |
| Online Access: | https://arxiv.org/abs/2307.06997 |
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Table of Contents:
- Moiré superlattices in stacked 2D crystals are powerful platforms for engineering correlated and topological quantum phases, with twisted graphene and transition metal dichalcogenides (TMDs) as prominent examples. Their angle-sensitive band structures enable rich tunability; however, conventional tear-and-stack methods fix the angle at assembly, limiting systematic exploration of angle-dependent phenomena. Here, we present a scanning-probe-based manipulation scheme that enables in situ, continuous post-fabrication twist control using nanostructured metal rotors. We demonstrate reproducible angle tuning and direct moiré imaging across three platforms: graphene, hBN, and encapsulated, air-sensitive MoTe2. Quantitative piezoresponse force microscopy (PFM) analysis confirms sub-degree precision with minimal induced heterostrain, preserving sample quality even in the marginally twisted regime. Crucially, the device architecture maintains open access to the active region, allowing optical, scanning-probe, and transport measurements. This work enables single-device mapping of the angular phase diagram of moiré materials, including the twisted TMD homobilayers.