Large circular photogalvanic effect in the noncentrosymmetric magnetic Weyl semimetal CeAlSi

Fuente: arXiv
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Main Authors: Karmakar, Abhirup Roy, Taraphder, A., Das, G. P.
Format: Preprint
Published: 2023
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author Karmakar, Abhirup Roy
Taraphder, A.
Das, G. P.
author_facet Karmakar, Abhirup Roy
Taraphder, A.
Das, G. P.
contents The recent discovery of the Weyl semimetal CeAlSi with simultaneous breaking of inversion and time-reversal symmetries has opened up new avenues for research into the interaction between light and topologically protected bands. In this work, we present a comprehensive examination of the shift current and injection current responsible for the circular photogalvanic effect in CeAlSi using first-principles calculations. Our investigation identifies a significant injection current of 4 mA/V$^2$ over a broad range in the near-infrared region of the electromagnetic spectrum, exceeding previously reported findings. In addition, we explored several externally controllable parameters to further enhance the photocurrent. A substantial boost in the injection current is observed when applying uniaxial strain along the $c$ axis of the crystal: a 5% strain results in a remarkable 64% increment. The exceptional photocurrent response in CeAlSi suggests that magnetic non-centrosymmetric Weyl semimetals may provide promising opportunities for novel photogalvanic applications.
format Preprint
id arxiv_https___arxiv_org_abs_2308_00045
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Large circular photogalvanic effect in the noncentrosymmetric magnetic Weyl semimetal CeAlSi
Karmakar, Abhirup Roy
Taraphder, A.
Das, G. P.
Mesoscale and Nanoscale Physics
Materials Science
The recent discovery of the Weyl semimetal CeAlSi with simultaneous breaking of inversion and time-reversal symmetries has opened up new avenues for research into the interaction between light and topologically protected bands. In this work, we present a comprehensive examination of the shift current and injection current responsible for the circular photogalvanic effect in CeAlSi using first-principles calculations. Our investigation identifies a significant injection current of 4 mA/V$^2$ over a broad range in the near-infrared region of the electromagnetic spectrum, exceeding previously reported findings. In addition, we explored several externally controllable parameters to further enhance the photocurrent. A substantial boost in the injection current is observed when applying uniaxial strain along the $c$ axis of the crystal: a 5% strain results in a remarkable 64% increment. The exceptional photocurrent response in CeAlSi suggests that magnetic non-centrosymmetric Weyl semimetals may provide promising opportunities for novel photogalvanic applications.
title Large circular photogalvanic effect in the noncentrosymmetric magnetic Weyl semimetal CeAlSi
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2308.00045