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Bibliographic Details
Main Authors: Mitsumoto, Kota, Takae, Kyohei
Format: Preprint
Published: 2023
Subjects:
Online Access:https://arxiv.org/abs/2308.04651
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Table of Contents:
  • We numerically show that molecules adsorbed in a soft porous crystal form a superlattice (SL) stabilized by elastic interactions. In a mechanically flexible honeycomb lattice model, when the elastic interactions between the next nearest neighboring lattice sites are strong, a long-range ordered 1/3-filling SL state emerges. By calculating the thermodynamic stability, it is found that the SL state is robust against thermal fluctuation. Our results provide a mechanism of elasticity-driven SL formation, which can be utilized for controlling the distribution of adsorbed molecules.