High mobility transport in isotopically-enriched $^{12}$C and $^{13}$C exfoliated graphene

Fuente: arXiv
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Main Authors: Iwakiri, Shuichi, Miller, Jakob, Lang, Florian, Prettenthaler, Jakob, Taniguchi, Takashi, Watanabe, Kenji, Lee, Sung Sik, Becker, Pascal, Günther, Detlef, Ihn, Thomas, Ensslin, Klaus
Format: Preprint
Published: 2023
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author Iwakiri, Shuichi
Miller, Jakob
Lang, Florian
Prettenthaler, Jakob
Taniguchi, Takashi
Watanabe, Kenji
Lee, Sung Sik
Becker, Pascal
Günther, Detlef
Ihn, Thomas
Ensslin, Klaus
author_facet Iwakiri, Shuichi
Miller, Jakob
Lang, Florian
Prettenthaler, Jakob
Taniguchi, Takashi
Watanabe, Kenji
Lee, Sung Sik
Becker, Pascal
Günther, Detlef
Ihn, Thomas
Ensslin, Klaus
contents Graphene quantum dots are promising candidates for qubits due to weak spin-orbit and hyperfine interactions. The hyperfine interaction, controllable via isotopic purification, could be the key to further improving the coherence. Here, we use isotopically enriched graphite crystals of both $^{12}$C and $^{13}$C grown by high-pressure-high-temperature method to exfoliate graphene layers. We fabricated Hall bar devices and performed quantum transport measurements, revealing mobilities exceeding $10^{5}$$\textrm{cm}^{2}/Vs$ and a long mean free path of microns, which are as high as natural graphene. Shubnikov-de Haas oscillations, quantum Hall effect up to the filling factor of one, and Brown-Zak oscillations due to the alignment of hBN and graphene are observed thanks to the high mobility. These results constitute a material platform for physics and engineering of isotopically-enriched graphene qubits.
format Preprint
id arxiv_https___arxiv_org_abs_2308_08175
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle High mobility transport in isotopically-enriched $^{12}$C and $^{13}$C exfoliated graphene
Iwakiri, Shuichi
Miller, Jakob
Lang, Florian
Prettenthaler, Jakob
Taniguchi, Takashi
Watanabe, Kenji
Lee, Sung Sik
Becker, Pascal
Günther, Detlef
Ihn, Thomas
Ensslin, Klaus
Mesoscale and Nanoscale Physics
Materials Science
Graphene quantum dots are promising candidates for qubits due to weak spin-orbit and hyperfine interactions. The hyperfine interaction, controllable via isotopic purification, could be the key to further improving the coherence. Here, we use isotopically enriched graphite crystals of both $^{12}$C and $^{13}$C grown by high-pressure-high-temperature method to exfoliate graphene layers. We fabricated Hall bar devices and performed quantum transport measurements, revealing mobilities exceeding $10^{5}$$\textrm{cm}^{2}/Vs$ and a long mean free path of microns, which are as high as natural graphene. Shubnikov-de Haas oscillations, quantum Hall effect up to the filling factor of one, and Brown-Zak oscillations due to the alignment of hBN and graphene are observed thanks to the high mobility. These results constitute a material platform for physics and engineering of isotopically-enriched graphene qubits.
title High mobility transport in isotopically-enriched $^{12}$C and $^{13}$C exfoliated graphene
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2308.08175