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Main Authors: Paske, Terry, Guan, Yingdong, Wang, Chaoguo, Moore, Curtis, Mao, Zhiqiang, Gui, Xin
Format: Preprint
Published: 2023
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Online Access:https://arxiv.org/abs/2309.01177
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author Paske, Terry
Guan, Yingdong
Wang, Chaoguo
Moore, Curtis
Mao, Zhiqiang
Gui, Xin
author_facet Paske, Terry
Guan, Yingdong
Wang, Chaoguo
Moore, Curtis
Mao, Zhiqiang
Gui, Xin
contents We report the crystal growth and characterization of a rare-earth-containing material, Dy3.00(1)Pt2Sb4.48(2). This compound possesses a similar structure to the previously reported Y3Pt4Ge6, but lacks two layers of Pt atoms. Crystallographic disorder was found in Dy3.00(1)Pt2Sb4.48(2). Additionally, the Dy-Dy framework was found to have both square net and triangular lattices. Dy3.00(1)Pt2Sb4.48(2)8 was determined to be antiferromagnetically ordered around ~15 K while a competing antiferromagnetic sublattice also exists at lower temperature. Strong magnetic anisotropy was observed and several metamagnetic transitions were seen in the hysteresis loops. Furthermore, the Curie-Weiss fitting revealed unusually small effective moment of Dy, which is far below the expected value of Dy3+ (10.65 muB). This material might provide a new platform to study the relation between crystallographic disorder and magnetism.
format Preprint
id arxiv_https___arxiv_org_abs_2309_01177
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Crystallographic Disorder and Strong Magnetic Anisotropy in Dy3.1Pt2.0Sb3.8
Paske, Terry
Guan, Yingdong
Wang, Chaoguo
Moore, Curtis
Mao, Zhiqiang
Gui, Xin
Materials Science
We report the crystal growth and characterization of a rare-earth-containing material, Dy3.00(1)Pt2Sb4.48(2). This compound possesses a similar structure to the previously reported Y3Pt4Ge6, but lacks two layers of Pt atoms. Crystallographic disorder was found in Dy3.00(1)Pt2Sb4.48(2). Additionally, the Dy-Dy framework was found to have both square net and triangular lattices. Dy3.00(1)Pt2Sb4.48(2)8 was determined to be antiferromagnetically ordered around ~15 K while a competing antiferromagnetic sublattice also exists at lower temperature. Strong magnetic anisotropy was observed and several metamagnetic transitions were seen in the hysteresis loops. Furthermore, the Curie-Weiss fitting revealed unusually small effective moment of Dy, which is far below the expected value of Dy3+ (10.65 muB). This material might provide a new platform to study the relation between crystallographic disorder and magnetism.
title Crystallographic Disorder and Strong Magnetic Anisotropy in Dy3.1Pt2.0Sb3.8
topic Materials Science
url https://arxiv.org/abs/2309.01177