Coexistence of near-EF flat band and van Hove singularity in a two-phase superconductor

Fuente: arXiv
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Autori principali: Chen, Xuezhi, Wang, Le, Ishizuka, Jun, Nogaki, Kosuke, Cheng, Yiwei, Yang, Fazhi, Zhang, Renjie, Chen, Zhenhua, Zhu, Fangyuan, Yanase, Youichi, Lv, Baiqing, Huang, Yaobo
Natura: Preprint
Pubblicazione: 2023
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author Chen, Xuezhi
Wang, Le
Ishizuka, Jun
Nogaki, Kosuke
Cheng, Yiwei
Yang, Fazhi
Zhang, Renjie
Chen, Zhenhua
Zhu, Fangyuan
Yanase, Youichi
Lv, Baiqing
Huang, Yaobo
author_facet Chen, Xuezhi
Wang, Le
Ishizuka, Jun
Nogaki, Kosuke
Cheng, Yiwei
Yang, Fazhi
Zhang, Renjie
Chen, Zhenhua
Zhu, Fangyuan
Yanase, Youichi
Lv, Baiqing
Huang, Yaobo
contents In quantum many-body systems, particularly, the ones with large near-EF density states, like flat bands or van Hove singularity (VHS), electron correlations often give rise to rich phase diagrams with multiple coexisting/competing orders occurring at similar energy scales. The recently discovered locally noncentrosymmetric heavy fermion superconductor CeRh2As2 has stimulated extensive attention due to its unusual H-T phase diagram, consisting of two-phase superconductivity, antiferromagnetic order, and possible quadrupole-density wave orders. However, despite its great importance, the near-EF electronic structure remains experimentally elusive. Here, we provide this key information by combining soft X-ray and vacuum ultraviolet (VUV) angle-resolved photoemission spectroscopy measurements and atom-resolved DFT+U calculations. With bulk-sensitive soft X-rays, we reveal quasi-2D hole- and 3D electron- pockets with a pronounced nesting feature. Most importantly, we observe a symmetry-protected fourfold VHS coexisting with the Ce 4f flat bands near the EF, which, to the best of our knowledge, has never been reported before. Such a rare coexistence is expected to lead to a large density of states at the zone edge, enhancement in electron correlations, and a large upper critical field of the odd-parity superconducting phase. Uniquely, it will also result in a new type of f-VHS hybridization that alters the order and fine electronic structure of the symmetry-protected VHS and flat bands. These peculiarities offer important dimensions for understanding the reported rich phase diagram and are discussed as an origin of superconductivity with two phases. Our findings not only provide key insights into the nature of multiple phases in CeRh$_2$As$_2$, but also open up new prospects for exploring the novelties of many-body systems with f-VHS hybridization.
format Preprint
id arxiv_https___arxiv_org_abs_2309_05895
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Coexistence of near-EF flat band and van Hove singularity in a two-phase superconductor
Chen, Xuezhi
Wang, Le
Ishizuka, Jun
Nogaki, Kosuke
Cheng, Yiwei
Yang, Fazhi
Zhang, Renjie
Chen, Zhenhua
Zhu, Fangyuan
Yanase, Youichi
Lv, Baiqing
Huang, Yaobo
Strongly Correlated Electrons
Materials Science
Superconductivity
In quantum many-body systems, particularly, the ones with large near-EF density states, like flat bands or van Hove singularity (VHS), electron correlations often give rise to rich phase diagrams with multiple coexisting/competing orders occurring at similar energy scales. The recently discovered locally noncentrosymmetric heavy fermion superconductor CeRh2As2 has stimulated extensive attention due to its unusual H-T phase diagram, consisting of two-phase superconductivity, antiferromagnetic order, and possible quadrupole-density wave orders. However, despite its great importance, the near-EF electronic structure remains experimentally elusive. Here, we provide this key information by combining soft X-ray and vacuum ultraviolet (VUV) angle-resolved photoemission spectroscopy measurements and atom-resolved DFT+U calculations. With bulk-sensitive soft X-rays, we reveal quasi-2D hole- and 3D electron- pockets with a pronounced nesting feature. Most importantly, we observe a symmetry-protected fourfold VHS coexisting with the Ce 4f flat bands near the EF, which, to the best of our knowledge, has never been reported before. Such a rare coexistence is expected to lead to a large density of states at the zone edge, enhancement in electron correlations, and a large upper critical field of the odd-parity superconducting phase. Uniquely, it will also result in a new type of f-VHS hybridization that alters the order and fine electronic structure of the symmetry-protected VHS and flat bands. These peculiarities offer important dimensions for understanding the reported rich phase diagram and are discussed as an origin of superconductivity with two phases. Our findings not only provide key insights into the nature of multiple phases in CeRh$_2$As$_2$, but also open up new prospects for exploring the novelties of many-body systems with f-VHS hybridization.
title Coexistence of near-EF flat band and van Hove singularity in a two-phase superconductor
topic Strongly Correlated Electrons
Materials Science
Superconductivity
url https://arxiv.org/abs/2309.05895