Stable nanofacets in [111] tilt grain boundaries of face-centered cubic metals

Fuente: arXiv
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Main Authors: Brink, Tobias, Langenohl, Lena, Pemma, Swetha, Liebscher, Christian H., Dehm, Gerhard
Format: Preprint
Published: 2023
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_version_ 1866910513497112576
author Brink, Tobias
Langenohl, Lena
Pemma, Swetha
Liebscher, Christian H.
Dehm, Gerhard
author_facet Brink, Tobias
Langenohl, Lena
Pemma, Swetha
Liebscher, Christian H.
Dehm, Gerhard
contents Grain boundaries can dissociate into facets if that reduces their excess energy. This, however, introduces line defects at the facet junctions, which present a driving force to grow the facets in order to reduce the total number of junctions and thus the system's energy. Often, micrometer-sized facet lengths are observed and facet growth only arrests for kinetic reasons. So far, energetically stable, finite-sized facets have not been observed, even though theoretical stability conditions have already been proposed. Here, we show a case where nanometer-sized facets are indeed stable compared to longer facets in [111] tilt grain boundaries in Cu by atomistic simulation and transmission electron microscopy. The facet junctions lack a Burgers vector component, which is unusual, but which removes the main energy cost of facet junctions. Only attractive interactions via line forces remain, which result from a discontinuity of grain boundary excess stress at the junction. Atomistic simulations predict that the same phenomenon also occurs in at least Al and Ag.
format Preprint
id arxiv_https___arxiv_org_abs_2309_07595
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Stable nanofacets in [111] tilt grain boundaries of face-centered cubic metals
Brink, Tobias
Langenohl, Lena
Pemma, Swetha
Liebscher, Christian H.
Dehm, Gerhard
Materials Science
Grain boundaries can dissociate into facets if that reduces their excess energy. This, however, introduces line defects at the facet junctions, which present a driving force to grow the facets in order to reduce the total number of junctions and thus the system's energy. Often, micrometer-sized facet lengths are observed and facet growth only arrests for kinetic reasons. So far, energetically stable, finite-sized facets have not been observed, even though theoretical stability conditions have already been proposed. Here, we show a case where nanometer-sized facets are indeed stable compared to longer facets in [111] tilt grain boundaries in Cu by atomistic simulation and transmission electron microscopy. The facet junctions lack a Burgers vector component, which is unusual, but which removes the main energy cost of facet junctions. Only attractive interactions via line forces remain, which result from a discontinuity of grain boundary excess stress at the junction. Atomistic simulations predict that the same phenomenon also occurs in at least Al and Ag.
title Stable nanofacets in [111] tilt grain boundaries of face-centered cubic metals
topic Materials Science
url https://arxiv.org/abs/2309.07595