Light-to-heat conversion of optically trapped hot Brownian particles

Fuente: arXiv
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Autores principales: Ortiz-Rivero, Elisa, Orozco-Barrera, Sergio, Chatterjee, Hirak, Gonzalez-Gomez, Carlos D., Caro, Carlos, Garcia-Martin, Maria L., Haro-Gonzalez, Patricia, Rica, Raul A., Gamez, Francisco
Formato: Preprint
Publicado: 2023
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author Ortiz-Rivero, Elisa
Orozco-Barrera, Sergio
Chatterjee, Hirak
Gonzalez-Gomez, Carlos D.
Caro, Carlos
Garcia-Martin, Maria L.
Haro-Gonzalez, Patricia
Rica, Raul A.
Gamez, Francisco
author_facet Ortiz-Rivero, Elisa
Orozco-Barrera, Sergio
Chatterjee, Hirak
Gonzalez-Gomez, Carlos D.
Caro, Carlos
Garcia-Martin, Maria L.
Haro-Gonzalez, Patricia
Rica, Raul A.
Gamez, Francisco
contents Anisotropic hybrid nanostructures stand out as promising therapeutic agents in photothermal conversion-based treatments. Accordingly, understanding local heat generation mediated by light-to-heat conversion of absorbing multicomponent nanoparticles at the single particle level have both forthwith become a subject of broad and current interest. Nonetheless, evaluating reliable temperature profiles around a single trapped nanoparticle is challenging from all experimental, computational, and fundamental viewpoints. Committed to filling this gap, the heat generation of an anisotropic hybrid nanostructure is explored by means of two different experimental approaches from which the local temperature is measured in a direct or indirect way, all in the context of the hot Brownian motion theory. The results were compared with analytical results supported by the numerical computation of the wavelength-dependent absorption efficiencies in the discrete dipole approximation for scattering calculations, which has been here extended to inhomogeneous nanostructures. Overall, we provide a consistent and comprehensive view of the heat generation in optical traps of highly absorbing particles under the viewpoint of the hot Brownian motion theory.
format Preprint
id arxiv_https___arxiv_org_abs_2309_11866
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Light-to-heat conversion of optically trapped hot Brownian particles
Ortiz-Rivero, Elisa
Orozco-Barrera, Sergio
Chatterjee, Hirak
Gonzalez-Gomez, Carlos D.
Caro, Carlos
Garcia-Martin, Maria L.
Haro-Gonzalez, Patricia
Rica, Raul A.
Gamez, Francisco
Mesoscale and Nanoscale Physics
Applied Physics
Anisotropic hybrid nanostructures stand out as promising therapeutic agents in photothermal conversion-based treatments. Accordingly, understanding local heat generation mediated by light-to-heat conversion of absorbing multicomponent nanoparticles at the single particle level have both forthwith become a subject of broad and current interest. Nonetheless, evaluating reliable temperature profiles around a single trapped nanoparticle is challenging from all experimental, computational, and fundamental viewpoints. Committed to filling this gap, the heat generation of an anisotropic hybrid nanostructure is explored by means of two different experimental approaches from which the local temperature is measured in a direct or indirect way, all in the context of the hot Brownian motion theory. The results were compared with analytical results supported by the numerical computation of the wavelength-dependent absorption efficiencies in the discrete dipole approximation for scattering calculations, which has been here extended to inhomogeneous nanostructures. Overall, we provide a consistent and comprehensive view of the heat generation in optical traps of highly absorbing particles under the viewpoint of the hot Brownian motion theory.
title Light-to-heat conversion of optically trapped hot Brownian particles
topic Mesoscale and Nanoscale Physics
Applied Physics
url https://arxiv.org/abs/2309.11866