FeGe1-xSbx:a series of novel kagome metals with noncollinear antiferromagnetism

Fuente: arXiv
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Main Authors: Huang, Jiale, Shang, Chenglin, Qin, Jianfei, Pan, Feihao, Shi, Bingxian, Wang, Jinchen, Liu, Juanjuan, Xu, Daye, Zhang, Hongxia, Wang, Hongliang, Hao, Lijie, Cheng, Peng
Format: Preprint
Published: 2023
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author Huang, Jiale
Shang, Chenglin
Qin, Jianfei
Pan, Feihao
Shi, Bingxian
Wang, Jinchen
Liu, Juanjuan
Xu, Daye
Zhang, Hongxia
Wang, Hongliang
Hao, Lijie
Cheng, Peng
author_facet Huang, Jiale
Shang, Chenglin
Qin, Jianfei
Pan, Feihao
Shi, Bingxian
Wang, Jinchen
Liu, Juanjuan
Xu, Daye
Zhang, Hongxia
Wang, Hongliang
Hao, Lijie
Cheng, Peng
contents Kagome metals are important for exploring emergent phenomena due to the interplay between band topology and electron correlation.Motivated by the recent discovery of charge density wave in a kagome lattice antiferromagnetic FeGe,we investigate the impact of Sb doping on the structural,charge and magnetic order of FeGe.The charge density wave is rapidly suppressed by Sb doping(~1.5%) and the antiferromagnetic ordering temperature gradually shifts to 280K for FeGe0.7Sb0.3.For FeGe1-xSbx with x>0.1,crystal structures with slightly distorted Fe kagome lattice are formed.Their magnetic anisotropy has significant change,temperature driven spin-reorientation and field-induced spin-flop transition are identified from magnetization measurement.Interestingly,neutron diffraction reveals noncollinear antiferromagnetic structures widely exist below TN for all sample with x>0.1.This noncollinear magnetic orders could possibly be unconventional and resulted from onsite repulsion and filling condition of kagome flat band,as predicted by a recent theoretical work.
format Preprint
id arxiv_https___arxiv_org_abs_2309_16502
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle FeGe1-xSbx:a series of novel kagome metals with noncollinear antiferromagnetism
Huang, Jiale
Shang, Chenglin
Qin, Jianfei
Pan, Feihao
Shi, Bingxian
Wang, Jinchen
Liu, Juanjuan
Xu, Daye
Zhang, Hongxia
Wang, Hongliang
Hao, Lijie
Cheng, Peng
Strongly Correlated Electrons
Materials Science
Superconductivity
Kagome metals are important for exploring emergent phenomena due to the interplay between band topology and electron correlation.Motivated by the recent discovery of charge density wave in a kagome lattice antiferromagnetic FeGe,we investigate the impact of Sb doping on the structural,charge and magnetic order of FeGe.The charge density wave is rapidly suppressed by Sb doping(~1.5%) and the antiferromagnetic ordering temperature gradually shifts to 280K for FeGe0.7Sb0.3.For FeGe1-xSbx with x>0.1,crystal structures with slightly distorted Fe kagome lattice are formed.Their magnetic anisotropy has significant change,temperature driven spin-reorientation and field-induced spin-flop transition are identified from magnetization measurement.Interestingly,neutron diffraction reveals noncollinear antiferromagnetic structures widely exist below TN for all sample with x>0.1.This noncollinear magnetic orders could possibly be unconventional and resulted from onsite repulsion and filling condition of kagome flat band,as predicted by a recent theoretical work.
title FeGe1-xSbx:a series of novel kagome metals with noncollinear antiferromagnetism
topic Strongly Correlated Electrons
Materials Science
Superconductivity
url https://arxiv.org/abs/2309.16502