Magnetic field induces giant nonlinear optical response in Weyl semimetals

Fuente: arXiv
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Main Authors: Bednik, Grigory, Kozii, Vladyslav
Format: Preprint
Published: 2023
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author Bednik, Grigory
Kozii, Vladyslav
author_facet Bednik, Grigory
Kozii, Vladyslav
contents We study the second-order optical response of Weyl semimetals in the presence of a magnetic field. We consider an idealized model of a perfectly linear Weyl node and use the Kubo formula at zero temperature to calculate the intrinsic contribution to photocurrent and second harmonic generation conductivity components. We obtain exact analytical expressions applicable at arbitrary values of frequency, chemical potential, and magnetic field. Our results show that finite magnetic field significantly enhances the nonlinear optical response in semimetals, while magnetic resonances lead to divergences in nonlinear conductivity. In realistic systems, these singularities are regularized by a finite scattering rate, but result in pronounced peaks which can be detected experimentally, provided the system is clean and interactions are weak. We also perform a semiclassical calculation that complements and confirms our microscopic results at small magnetic fields and frequencies.
format Preprint
id arxiv_https___arxiv_org_abs_2310_02578
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Magnetic field induces giant nonlinear optical response in Weyl semimetals
Bednik, Grigory
Kozii, Vladyslav
Mesoscale and Nanoscale Physics
Materials Science
Strongly Correlated Electrons
We study the second-order optical response of Weyl semimetals in the presence of a magnetic field. We consider an idealized model of a perfectly linear Weyl node and use the Kubo formula at zero temperature to calculate the intrinsic contribution to photocurrent and second harmonic generation conductivity components. We obtain exact analytical expressions applicable at arbitrary values of frequency, chemical potential, and magnetic field. Our results show that finite magnetic field significantly enhances the nonlinear optical response in semimetals, while magnetic resonances lead to divergences in nonlinear conductivity. In realistic systems, these singularities are regularized by a finite scattering rate, but result in pronounced peaks which can be detected experimentally, provided the system is clean and interactions are weak. We also perform a semiclassical calculation that complements and confirms our microscopic results at small magnetic fields and frequencies.
title Magnetic field induces giant nonlinear optical response in Weyl semimetals
topic Mesoscale and Nanoscale Physics
Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2310.02578