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Hauptverfasser: Baek, Insu, Han, Seungyun, Cheon, Suik, Lee, Hyun-Woo
Format: Preprint
Veröffentlicht: 2023
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Online-Zugang:https://arxiv.org/abs/2310.05113
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author Baek, Insu
Han, Seungyun
Cheon, Suik
Lee, Hyun-Woo
author_facet Baek, Insu
Han, Seungyun
Cheon, Suik
Lee, Hyun-Woo
contents Nonlinear spintronics combines nonlinear dynamics with spintronics, opening up new possibilities beyond linear responses. A recent theoretical work [Xiao et al., Phys. Rev. Lett. 130, 166302 (2023)] predicts the nonlinear generation of spin density [nonlinear spin Edelstein effect (NSEE)] in centrosymmetric metals based on symmetry analysis combined with first principle calculation. However, its microscopic mechanism is limited to a specific set of materials with local inversion symmetry breaking and is not applicable to general materials. This paper focuses on the fundamental role of orbital degrees of freedom for the nonlinear generation in centrosymmetric systems. Using a combination of tight-binding model and density functional theory calculations, we demonstrate that nonlinear orbital density can arise independently of spin-orbit coupling. In contrast, spin density follows through spin-orbit coupling. We further elucidate the microscopic mechanism responsible for this phenomenon, which involves the NSEE induced by electric-field-induced orbital Rashba texture. In addition, we also explore the potential applications of the nonlinear orbital and spin Edelstein effect for field-free switching of magnetization.
format Preprint
id arxiv_https___arxiv_org_abs_2310_05113
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Nonlinear Orbital and Spin Edelstein Effect in Centrosymmetric Metals
Baek, Insu
Han, Seungyun
Cheon, Suik
Lee, Hyun-Woo
Materials Science
Nonlinear spintronics combines nonlinear dynamics with spintronics, opening up new possibilities beyond linear responses. A recent theoretical work [Xiao et al., Phys. Rev. Lett. 130, 166302 (2023)] predicts the nonlinear generation of spin density [nonlinear spin Edelstein effect (NSEE)] in centrosymmetric metals based on symmetry analysis combined with first principle calculation. However, its microscopic mechanism is limited to a specific set of materials with local inversion symmetry breaking and is not applicable to general materials. This paper focuses on the fundamental role of orbital degrees of freedom for the nonlinear generation in centrosymmetric systems. Using a combination of tight-binding model and density functional theory calculations, we demonstrate that nonlinear orbital density can arise independently of spin-orbit coupling. In contrast, spin density follows through spin-orbit coupling. We further elucidate the microscopic mechanism responsible for this phenomenon, which involves the NSEE induced by electric-field-induced orbital Rashba texture. In addition, we also explore the potential applications of the nonlinear orbital and spin Edelstein effect for field-free switching of magnetization.
title Nonlinear Orbital and Spin Edelstein Effect in Centrosymmetric Metals
topic Materials Science
url https://arxiv.org/abs/2310.05113