Inverse exciton spin orientation due to trion formation in modulation doped quantum wells

Fuente: arXiv
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Main Authors: Kotova, Lyubov, Platonov, Alexei, Kochereshko, Vladimir
Format: Preprint
Published: 2023
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author Kotova, Lyubov
Platonov, Alexei
Kochereshko, Vladimir
author_facet Kotova, Lyubov
Platonov, Alexei
Kochereshko, Vladimir
contents Time-resolved and time-integrated circularly polarized photoluminescence of excitons and trions in external magnetic fields up to 10 T has been studied in undoped and n-type doped quantum well structures based on ZnSe. In an undoped structure, a circular polarization of photoluminescence induced by magnetic fields corresponded to the Boltzmann distribution of excitons on Zeeman sublevels. The inverse spin orientation of excitons is observed in doped samples with a carrier density of $3 \times 10^{10}$ cm$^{-2}$ and higher. Model calculations show that the reason for the inverse spin orientation is the effective depletion of the lowest-exciton Zeeman sublevel as a result of the spin-dependent formation of trions. The trion formation time as a result of exciton-electron binding was determined as 2 ps. This is noticeably shorter than the characteristic time of the exciton-photon interaction. The observed effect can be considered as a way of spin manipulation by electric fields.
format Preprint
id arxiv_https___arxiv_org_abs_2310_06651
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Inverse exciton spin orientation due to trion formation in modulation doped quantum wells
Kotova, Lyubov
Platonov, Alexei
Kochereshko, Vladimir
Mesoscale and Nanoscale Physics
Time-resolved and time-integrated circularly polarized photoluminescence of excitons and trions in external magnetic fields up to 10 T has been studied in undoped and n-type doped quantum well structures based on ZnSe. In an undoped structure, a circular polarization of photoluminescence induced by magnetic fields corresponded to the Boltzmann distribution of excitons on Zeeman sublevels. The inverse spin orientation of excitons is observed in doped samples with a carrier density of $3 \times 10^{10}$ cm$^{-2}$ and higher. Model calculations show that the reason for the inverse spin orientation is the effective depletion of the lowest-exciton Zeeman sublevel as a result of the spin-dependent formation of trions. The trion formation time as a result of exciton-electron binding was determined as 2 ps. This is noticeably shorter than the characteristic time of the exciton-photon interaction. The observed effect can be considered as a way of spin manipulation by electric fields.
title Inverse exciton spin orientation due to trion formation in modulation doped quantum wells
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2310.06651