Magnetic structure, excitations and field induced transitions in the honeycomb lattice $\rm{Er_2Si_2O_7}$

Fuente: arXiv
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Autori principali: Islam, M., d'Ambrumenil, N., Khalyavin, D. D., Manuel, P., Orlandi, F., Ollivier, J., Hatnean, M. Ciomaga, Balakrishnan, G., Petrenko, O. A.
Natura: Preprint
Pubblicazione: 2023
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author Islam, M.
d'Ambrumenil, N.
Khalyavin, D. D.
Manuel, P.
Orlandi, F.
Ollivier, J.
Hatnean, M. Ciomaga
Balakrishnan, G.
Petrenko, O. A.
author_facet Islam, M.
d'Ambrumenil, N.
Khalyavin, D. D.
Manuel, P.
Orlandi, F.
Ollivier, J.
Hatnean, M. Ciomaga
Balakrishnan, G.
Petrenko, O. A.
contents We investigate the magnetic properties of the monoclinic D-type $\rm{Er_2Si_2O_7}$ with a distorted honeycomb lattice using powder and single crystal neutron scattering techniques, as well as single crystal magnetisation measurements. The powder neutron diffraction shows that below the ordering temperature, $T_{\rm N}=1.85$ K, the compound forms a ${\bf q}=0$ antiferromagnetic structure with four sublattices. For $H \! \parallel \! a$, magnetisation measurements reveal a narrow, but clearly visible plateau at one third of the magnetisation saturation value. The plateau's stabilisation is accompanied by a significant increase of the magnetic unit cell, as the magnetic peaks with fractional indices are observed in single crystal neutron diffraction experiments. At low-temperatures, the inelastic neutron scattering measurements reveal the presence of low-energy dispersionless excitations. Their spectrum is sensitive to the applied field, it significantly softens on the magnetisation plateau, and demonstrates the behaviour expected for a non-collinear Ising antiferromagnet away from the plateau.
format Preprint
id arxiv_https___arxiv_org_abs_2310_09268
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Magnetic structure, excitations and field induced transitions in the honeycomb lattice $\rm{Er_2Si_2O_7}$
Islam, M.
d'Ambrumenil, N.
Khalyavin, D. D.
Manuel, P.
Orlandi, F.
Ollivier, J.
Hatnean, M. Ciomaga
Balakrishnan, G.
Petrenko, O. A.
Strongly Correlated Electrons
We investigate the magnetic properties of the monoclinic D-type $\rm{Er_2Si_2O_7}$ with a distorted honeycomb lattice using powder and single crystal neutron scattering techniques, as well as single crystal magnetisation measurements. The powder neutron diffraction shows that below the ordering temperature, $T_{\rm N}=1.85$ K, the compound forms a ${\bf q}=0$ antiferromagnetic structure with four sublattices. For $H \! \parallel \! a$, magnetisation measurements reveal a narrow, but clearly visible plateau at one third of the magnetisation saturation value. The plateau's stabilisation is accompanied by a significant increase of the magnetic unit cell, as the magnetic peaks with fractional indices are observed in single crystal neutron diffraction experiments. At low-temperatures, the inelastic neutron scattering measurements reveal the presence of low-energy dispersionless excitations. Their spectrum is sensitive to the applied field, it significantly softens on the magnetisation plateau, and demonstrates the behaviour expected for a non-collinear Ising antiferromagnet away from the plateau.
title Magnetic structure, excitations and field induced transitions in the honeycomb lattice $\rm{Er_2Si_2O_7}$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2310.09268