Identification of electronic dimensionality reduction in semiconductor quantum well structures

Fuente: arXiv
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Main Authors: Takeda, Takahito, Takase, Kengo, Strocov, Vladimir N., Tanaka, Masaaki, Kobayashi, Masaki
Format: Preprint
Published: 2023
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author Takeda, Takahito
Takase, Kengo
Strocov, Vladimir N.
Tanaka, Masaaki
Kobayashi, Masaki
author_facet Takeda, Takahito
Takase, Kengo
Strocov, Vladimir N.
Tanaka, Masaaki
Kobayashi, Masaki
contents Two-dimensional (2D) systems, such as high-temperature superconductors, surface states of topological insulators, and layered materials, have been intensively studied using vacuum-ultraviolet (VUV) angle-resolved photoemission spectroscopy (ARPES). In semiconductor films (heterostructures), quantum well (QW) states arise due to electron/hole accumulations at the surface (interface). The quantized states due to quantum confinement can be observed by VUV-ARPES, while the periodic intensity modulations along the surface normal (kz) direction of these quantized states are also observable by varying incident photon energy, resembling three-dimensional (3D) band dispersion. We have conducted soft X-ray (SX) ARPES measurements on thick and ultrathin III-V semiconductor InSb(001) films to investigate the electronic dimensionality reduction in semiconductor QWs. In addition to the dissipation of the kz dispersion, the SX-ARPES observations demonstrate the changes of the symmetry and periodicity of the Brillouin zone in the ultrathin film as 2D QW compared with these of the 3D bulk one, indicating the electronic dimensionality reduction of the 3D bulk band dispersion caused by the quantum confinement. The results provide a critical diagnosis using SX-ARPES for the dimensionality reduction in semiconductor QW structures.
format Preprint
id arxiv_https___arxiv_org_abs_2310_12423
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Identification of electronic dimensionality reduction in semiconductor quantum well structures
Takeda, Takahito
Takase, Kengo
Strocov, Vladimir N.
Tanaka, Masaaki
Kobayashi, Masaki
Materials Science
Two-dimensional (2D) systems, such as high-temperature superconductors, surface states of topological insulators, and layered materials, have been intensively studied using vacuum-ultraviolet (VUV) angle-resolved photoemission spectroscopy (ARPES). In semiconductor films (heterostructures), quantum well (QW) states arise due to electron/hole accumulations at the surface (interface). The quantized states due to quantum confinement can be observed by VUV-ARPES, while the periodic intensity modulations along the surface normal (kz) direction of these quantized states are also observable by varying incident photon energy, resembling three-dimensional (3D) band dispersion. We have conducted soft X-ray (SX) ARPES measurements on thick and ultrathin III-V semiconductor InSb(001) films to investigate the electronic dimensionality reduction in semiconductor QWs. In addition to the dissipation of the kz dispersion, the SX-ARPES observations demonstrate the changes of the symmetry and periodicity of the Brillouin zone in the ultrathin film as 2D QW compared with these of the 3D bulk one, indicating the electronic dimensionality reduction of the 3D bulk band dispersion caused by the quantum confinement. The results provide a critical diagnosis using SX-ARPES for the dimensionality reduction in semiconductor QW structures.
title Identification of electronic dimensionality reduction in semiconductor quantum well structures
topic Materials Science
url https://arxiv.org/abs/2310.12423