Spectral stability of V2 centres in sub-micron 4H-SiC membranes

Fuente: arXiv
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Main Authors: Heiler, Jonah, Körber, Jonathan, Hesselmeier, Erik, Kuna, Pierre, Stöhr, Rainer, Fuchs, Philipp, Ghezellou, Misagh, Ul-Hassan, Jawad, Knolle, Wolfgang, Becher, Christoph, Kaiser, Florian, Wrachtrup, Jörg
Format: Preprint
Published: 2023
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author Heiler, Jonah
Körber, Jonathan
Hesselmeier, Erik
Kuna, Pierre
Stöhr, Rainer
Fuchs, Philipp
Ghezellou, Misagh
Ul-Hassan, Jawad
Knolle, Wolfgang
Becher, Christoph
Kaiser, Florian
Wrachtrup, Jörg
author_facet Heiler, Jonah
Körber, Jonathan
Hesselmeier, Erik
Kuna, Pierre
Stöhr, Rainer
Fuchs, Philipp
Ghezellou, Misagh
Ul-Hassan, Jawad
Knolle, Wolfgang
Becher, Christoph
Kaiser, Florian
Wrachtrup, Jörg
contents Colour centres in silicon carbide emerge as a promising semiconductor quantum technology platform with excellent spin-optical coherences.However, recent efforts towards maximising the photonic efficiency via integration into nanophotonic structures proved to be challenging due to reduced spectral stabilities. Here, we provide a large-scale systematic investigation on silicon vacancy centres in thin silicon carbide membranes with thicknesses down to $0.25\,\rmμm$. Our membrane fabrication process involves a combination of chemical mechanical polishing, reactive ion etching, and subsequent annealing. This leads to highly reproducible membranes with roughness values of $3-4\,\rmÅ$, as well as negligible surface fluorescence. We find that silicon vacancy centres show close-to lifetime limited optical linewidths with almost no signs of spectral wandering down to membrane thicknesses of $0.7 \,\rmμm$. For silicon vacancy centres in thinner membranes down to $0.25\,\rmμm$, we observe spectral wandering, however, optical linewidths remain below $200\,\rm MHz$, which is compatible with spin-selective excitation schemes. Our work clearly shows that silicon vacancy centres can be integrated into sub-micron silicon carbide membranes, which opens the avenue towards obtaining the necessary improvements in photon extraction efficiency based on nanophotonic structuring.
format Preprint
id arxiv_https___arxiv_org_abs_2310_12617
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Spectral stability of V2 centres in sub-micron 4H-SiC membranes
Heiler, Jonah
Körber, Jonathan
Hesselmeier, Erik
Kuna, Pierre
Stöhr, Rainer
Fuchs, Philipp
Ghezellou, Misagh
Ul-Hassan, Jawad
Knolle, Wolfgang
Becher, Christoph
Kaiser, Florian
Wrachtrup, Jörg
Quantum Physics
Optics
Colour centres in silicon carbide emerge as a promising semiconductor quantum technology platform with excellent spin-optical coherences.However, recent efforts towards maximising the photonic efficiency via integration into nanophotonic structures proved to be challenging due to reduced spectral stabilities. Here, we provide a large-scale systematic investigation on silicon vacancy centres in thin silicon carbide membranes with thicknesses down to $0.25\,\rmμm$. Our membrane fabrication process involves a combination of chemical mechanical polishing, reactive ion etching, and subsequent annealing. This leads to highly reproducible membranes with roughness values of $3-4\,\rmÅ$, as well as negligible surface fluorescence. We find that silicon vacancy centres show close-to lifetime limited optical linewidths with almost no signs of spectral wandering down to membrane thicknesses of $0.7 \,\rmμm$. For silicon vacancy centres in thinner membranes down to $0.25\,\rmμm$, we observe spectral wandering, however, optical linewidths remain below $200\,\rm MHz$, which is compatible with spin-selective excitation schemes. Our work clearly shows that silicon vacancy centres can be integrated into sub-micron silicon carbide membranes, which opens the avenue towards obtaining the necessary improvements in photon extraction efficiency based on nanophotonic structuring.
title Spectral stability of V2 centres in sub-micron 4H-SiC membranes
topic Quantum Physics
Optics
url https://arxiv.org/abs/2310.12617