Nonrelativistic spin splittings and altermagnetism in twisted bilayers of centrosymmetric antiferromagnets

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Autori principali: Sheoran, Sajjan, Bhattacharya, Saswata
Natura: Preprint
Pubblicazione: 2023
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author Sheoran, Sajjan
Bhattacharya, Saswata
author_facet Sheoran, Sajjan
Bhattacharya, Saswata
contents Magnetism-driven nonrelativistic spin splittings (NRSS) are promising for highly efficient spintronics applications. Although 2D centrosymmetric (in four-dimensional spacetime) antiferromagnets are abundant, they have not received extensive research attention owing to symmetry-forbidden spin polarization and magnetization. Here, we demonstrate a paradigm to harness NRSS by twisting the bilayer of centrosymmetric antiferromagnets with commensurate twist angles. We observe $i$-wave altermagnetism and spin-momentum locking by first-principles simulations and symmetry analysis on prototypical MnPSe$_3$ and MnSe antiferromagnets. The strength of NRSS (up to 80 meVÅ) induced by twisting is comparable to SOC-induced linear Rashba-Dresselhaus effects. The results also demonstrate how applying biaxial strain and a vertical electric field tune the NRSS. The findings reveal the untapped potential of centrosymmetric antiferromagnets and thus expand the material's horizons in spintronics.
format Preprint
id arxiv_https___arxiv_org_abs_2310_19395
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Nonrelativistic spin splittings and altermagnetism in twisted bilayers of centrosymmetric antiferromagnets
Sheoran, Sajjan
Bhattacharya, Saswata
Materials Science
Mesoscale and Nanoscale Physics
Magnetism-driven nonrelativistic spin splittings (NRSS) are promising for highly efficient spintronics applications. Although 2D centrosymmetric (in four-dimensional spacetime) antiferromagnets are abundant, they have not received extensive research attention owing to symmetry-forbidden spin polarization and magnetization. Here, we demonstrate a paradigm to harness NRSS by twisting the bilayer of centrosymmetric antiferromagnets with commensurate twist angles. We observe $i$-wave altermagnetism and spin-momentum locking by first-principles simulations and symmetry analysis on prototypical MnPSe$_3$ and MnSe antiferromagnets. The strength of NRSS (up to 80 meVÅ) induced by twisting is comparable to SOC-induced linear Rashba-Dresselhaus effects. The results also demonstrate how applying biaxial strain and a vertical electric field tune the NRSS. The findings reveal the untapped potential of centrosymmetric antiferromagnets and thus expand the material's horizons in spintronics.
title Nonrelativistic spin splittings and altermagnetism in twisted bilayers of centrosymmetric antiferromagnets
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2310.19395