Optical pumping of ${\mathrm{5s4d} ^1\mathrm{D}_2}$ strontium atoms for laser cooling and imaging

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Auteurs principaux: Samland, Jens, Bennetts, Shayne, Chen, Chun-Chia, Escudero, Rodrigo González, Schreck, Florian, Pasquiou, Benjamin
Format: Preprint
Publié: 2023
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author Samland, Jens
Bennetts, Shayne
Chen, Chun-Chia
Escudero, Rodrigo González
Schreck, Florian
Pasquiou, Benjamin
author_facet Samland, Jens
Bennetts, Shayne
Chen, Chun-Chia
Escudero, Rodrigo González
Schreck, Florian
Pasquiou, Benjamin
contents We present a faster repumping scheme for strontium magneto-optical traps operating on the broad ${\mathrm{5s^2} ^1\mathrm{S}_0} - {\mathrm{5s5p} ^1\mathrm{P}_1}$ laser cooling transition. Contrary to existing repumping schemes, we directly address lost atoms that spontaneously decayed to the ${\mathrm{5s4d} ^1\mathrm{D}_2}$ state, sending them back into the laser cooling cycle by optical pumping on the ${\mathrm{5s4d} ^1\mathrm{D}_2} - {\mathrm{5s8p} ^1\mathrm{P}_1}$ transition. We thus avoid the $\sim 100 \, \mathrm{μs}$-slow decay path from ${\mathrm{5s4d} ^1\mathrm{D}_2}$ to the ${\mathrm{5s5p} ^3\mathrm{P}_{1,2}}$ states that is part of other repumping schemes. Using one low-cost external-cavity diode laser emitting at $448 \, \mathrm{nm}$, we show our scheme increases the flux out of a 2D magneto-optical trap by $60 \, \%$ compared to without repumping. Furthermore, we perform spectroscopy on the ${\mathrm{5s4d} ^1\mathrm{D}_2} - {\mathrm{5s8p} ^1\mathrm{P}_1}$ transition and measure its frequency $ν_{\mathrm{^{88}Sr}} = (668917515.3 \pm 4.0 \pm 25) \, \mathrm{MHz}$. We also measure the frequency shifts between the four stable isotopes of strontium and infer the specific mass and field shift factors, $δν_\text{SMS} ^{88,86} = -267(45) \, \mathrm{MHz}$ and $δν_\text{FS} ^{88,86} = 2(42) \, \mathrm{MHz}$. Finally, we measure the hyperfine splitting of the ${\mathrm{5s8p} ^1\mathrm{P}_1}$ state in fermionic strontium, and deduce the magnetic dipole and electric quadrupole coupling coefficients $A = -4(5) \, \mathrm{MHz}$ and $B = 5(35) \, \mathrm{MHz}$. Our experimental demonstration shows that this simple and very fast scheme could improve the laser cooling and imaging performance of cold strontium atom devices, such as quantum computers based on strontium atoms in arrays of optical tweezers.
format Preprint
id arxiv_https___arxiv_org_abs_2311_02941
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Optical pumping of ${\mathrm{5s4d} ^1\mathrm{D}_2}$ strontium atoms for laser cooling and imaging
Samland, Jens
Bennetts, Shayne
Chen, Chun-Chia
Escudero, Rodrigo González
Schreck, Florian
Pasquiou, Benjamin
Atomic Physics
We present a faster repumping scheme for strontium magneto-optical traps operating on the broad ${\mathrm{5s^2} ^1\mathrm{S}_0} - {\mathrm{5s5p} ^1\mathrm{P}_1}$ laser cooling transition. Contrary to existing repumping schemes, we directly address lost atoms that spontaneously decayed to the ${\mathrm{5s4d} ^1\mathrm{D}_2}$ state, sending them back into the laser cooling cycle by optical pumping on the ${\mathrm{5s4d} ^1\mathrm{D}_2} - {\mathrm{5s8p} ^1\mathrm{P}_1}$ transition. We thus avoid the $\sim 100 \, \mathrm{μs}$-slow decay path from ${\mathrm{5s4d} ^1\mathrm{D}_2}$ to the ${\mathrm{5s5p} ^3\mathrm{P}_{1,2}}$ states that is part of other repumping schemes. Using one low-cost external-cavity diode laser emitting at $448 \, \mathrm{nm}$, we show our scheme increases the flux out of a 2D magneto-optical trap by $60 \, \%$ compared to without repumping. Furthermore, we perform spectroscopy on the ${\mathrm{5s4d} ^1\mathrm{D}_2} - {\mathrm{5s8p} ^1\mathrm{P}_1}$ transition and measure its frequency $ν_{\mathrm{^{88}Sr}} = (668917515.3 \pm 4.0 \pm 25) \, \mathrm{MHz}$. We also measure the frequency shifts between the four stable isotopes of strontium and infer the specific mass and field shift factors, $δν_\text{SMS} ^{88,86} = -267(45) \, \mathrm{MHz}$ and $δν_\text{FS} ^{88,86} = 2(42) \, \mathrm{MHz}$. Finally, we measure the hyperfine splitting of the ${\mathrm{5s8p} ^1\mathrm{P}_1}$ state in fermionic strontium, and deduce the magnetic dipole and electric quadrupole coupling coefficients $A = -4(5) \, \mathrm{MHz}$ and $B = 5(35) \, \mathrm{MHz}$. Our experimental demonstration shows that this simple and very fast scheme could improve the laser cooling and imaging performance of cold strontium atom devices, such as quantum computers based on strontium atoms in arrays of optical tweezers.
title Optical pumping of ${\mathrm{5s4d} ^1\mathrm{D}_2}$ strontium atoms for laser cooling and imaging
topic Atomic Physics
url https://arxiv.org/abs/2311.02941