Tuning Multipolar Mie Scattering of Particles on a Dielectric-Covered Mirror

Fuente: arXiv
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Auteurs principaux: Yao, Kan, Fang, Jie, Jiang, Taizhi, Briggs, Andrew F., Skipper, Alec M., Kim, Youngsun, Belkin, Mikhail A., Korgel, Brian A., Bank, Seth R., Zheng, Yuebing
Format: Preprint
Publié: 2023
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author Yao, Kan
Fang, Jie
Jiang, Taizhi
Briggs, Andrew F.
Skipper, Alec M.
Kim, Youngsun
Belkin, Mikhail A.
Korgel, Brian A.
Bank, Seth R.
Zheng, Yuebing
author_facet Yao, Kan
Fang, Jie
Jiang, Taizhi
Briggs, Andrew F.
Skipper, Alec M.
Kim, Youngsun
Belkin, Mikhail A.
Korgel, Brian A.
Bank, Seth R.
Zheng, Yuebing
contents Optically resonant particles are key building blocks of many nanophotonic devices such as optical antennas and metasurfaces. Because the functionalities of such devices are largely determined by the optical properties of individual resonators, extending the attainable responses from a given particle is highly desirable. Practically, this is usually achieved by introducing an asymmetric dielectric environment. However, commonly used simple substrates have limited influences on the optical properties of the particles atop. Here, we show that the multipolar scattering of silicon microspheres can be effectively modified by placing the particles on a dielectric-covered mirror, which tunes the coupling between the Mie resonances of microspheres and the standing waves and waveguide modes in the dielectric spacer. This tunability allows selective excitation, enhancement, and suppression of the multipolar resonances and enables scattering at extended wavelengths, providing new opportunities in controlling light-matter interactions for various applications. We further demonstrate with experiments the detection of molecular fingerprints by single-particle mid-infrared spectroscopy, and, with simulations strong optical repulsive forces that could elevate the particles from a substrate.
format Preprint
id arxiv_https___arxiv_org_abs_2311_06488
institution arXiv
publishDate 2023
record_format arxiv
spellingShingle Tuning Multipolar Mie Scattering of Particles on a Dielectric-Covered Mirror
Yao, Kan
Fang, Jie
Jiang, Taizhi
Briggs, Andrew F.
Skipper, Alec M.
Kim, Youngsun
Belkin, Mikhail A.
Korgel, Brian A.
Bank, Seth R.
Zheng, Yuebing
Optics
Applied Physics
Optically resonant particles are key building blocks of many nanophotonic devices such as optical antennas and metasurfaces. Because the functionalities of such devices are largely determined by the optical properties of individual resonators, extending the attainable responses from a given particle is highly desirable. Practically, this is usually achieved by introducing an asymmetric dielectric environment. However, commonly used simple substrates have limited influences on the optical properties of the particles atop. Here, we show that the multipolar scattering of silicon microspheres can be effectively modified by placing the particles on a dielectric-covered mirror, which tunes the coupling between the Mie resonances of microspheres and the standing waves and waveguide modes in the dielectric spacer. This tunability allows selective excitation, enhancement, and suppression of the multipolar resonances and enables scattering at extended wavelengths, providing new opportunities in controlling light-matter interactions for various applications. We further demonstrate with experiments the detection of molecular fingerprints by single-particle mid-infrared spectroscopy, and, with simulations strong optical repulsive forces that could elevate the particles from a substrate.
title Tuning Multipolar Mie Scattering of Particles on a Dielectric-Covered Mirror
topic Optics
Applied Physics
url https://arxiv.org/abs/2311.06488